Mean-field model of interacting quasilocalized excitations in glasses

被引:25
|
作者
Rainone, Corrado [1 ]
Urbani, Pierfrancesco [2 ]
Zamponi, Francesco [3 ]
Lerner, Edan [1 ]
Bouchbinder, Eran [4 ]
机构
[1] Univ Amsterdam, Inst Theoret Phys, Sci Pk 904, Amsterdam, Netherlands
[2] Univ Paris Saclay, Inst Phys Theor, CNRS, CEA, F-91191 Gif Sur Yvette, France
[3] Univ Paris, Sorbonne Univ, Univ PSL, Lab Phys,Ecole Normale Super,CNRS,ENS, F-75005 Paris, France
[4] Weizmann Inst Sci, Chem & Biol Phys Dept, IL-7610001 Rehovot, Israel
来源
SCIPOST PHYSICS CORE | 2021年 / 4卷 / 02期
基金
欧洲研究理事会;
关键词
INSTANTANEOUS NORMAL-MODES; SUPERCOOLED LIQUID; SOFT;
D O I
10.21468/SciPostPhysCore.4.2.008
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Structural glasses feature quasilocalized excitations whose frequencies omega follow a universal density of states D(omega)similar to omega(4). Yet, the underlying physics behind this universality is not fully understood. Here we study a mean-field model of quasilocalized excitations in glasses, viewed as groups of particles embedded inside an elastic medium and described collectively as anharmonic oscillators. The oscillators, whose harmonic stiffness is taken from a rather featureless probability distribution (of upper cutoff kappa(0)) in the absence of interactions, interact among themselves through random couplings (characterized by a strength J) and with the surrounding elastic medium (an interaction characterized by a constant force h). We first show that the model gives rise to a gapless density of states D(omega) = A(g) omega(4) for a broad range of model parameters, expressed in terms of the strength of the oscillators' stabilizing anharmonicity, which plays a decisive role in the model. Then - using scaling theory and numerical simulations - we provide a complete understanding of the non-universal prefactor A(g) (h, J, kappa(0)), of the oscillators' interaction-induced mean square displacement and of an emerging characteristic frequency, all in terms of properly identified dimensionless quantities. In particular, we show that A(g) (h, J, kappa(0)) is a non-monotonic function of J for a fixed h, varying predominantly exponentially with -(kappa(0)h(2/3)/J(2)) in the weak interactions (small J) regime reminiscent of recent observations in computer glasses - and predominantly decays as a power-law for larger J, in a regime where h plays no role. We discuss the physical interpretation of the model and its possible relations to available observations in structural glasses, along with delineating some future research directions.
引用
收藏
页数:15
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