Direct decomposition of NO by microwave heating over Fe/NaZSM-5

被引:62
作者
Tang, JW [1 ]
Zhang, T [1 ]
Liang, DB [1 ]
Yang, HH [1 ]
Li, N [1 ]
Lin, LW [1 ]
机构
[1] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
关键词
NO decomposition; microwave heating; Fe/NaZSM-5; O-2; endurance;
D O I
10.1016/S0926-3373(01)00268-5
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Catalytic decomposition of NO was studied over Fe/NaZSM-5 catalyst. Novel results were observed with the microwave heating mode. The conversion of NO to N-2 increased remarkably with the increasing of Fe loading. The effects of a series of reaction parameters, including reaction temperature, O-2 concentration, NO concentration, gas flow rate and H2O addition, on the productivity of N-2 have been investigated. It is shown that the catalyst exhibited good endurance to excess O-2 in the microwave heating mode. Under all reaction conditions, NO converted predominantly to N-2. The highest conversion of NO to N-2 was up to 70%. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:1 / 7
页数:7
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