225Ac and 223Ra production via 800 MeV proton irradiation of natural thorium targets

被引:68
作者
Weidner, J. W. [1 ]
Mashnik, S. G. [1 ]
John, K. D. [1 ]
Ballard, B. [1 ]
Birnbaum, E. R. [1 ]
Bitteker, L. J. [1 ]
Couture, A. [1 ]
Fassbender, M. E. [1 ]
Goff, G. S. [1 ]
Gritzo, R. [1 ]
Hemez, F. M. [1 ]
Runde, W. [1 ]
Ullmann, J. L. [1 ]
Wolfsberg, L. E. [1 ]
Nortier, F. M. [1 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
基金
美国能源部;
关键词
Actinium-225; Radium-223; Cross section; Yield; Proton irradiation; Thorium target; TOTAL CROSS-SECTIONS; ENERGY-RANGE; NA-22; THERAPY; BE-7; RADIOIMMUNOTHERAPY; ACTINIUM-225; AL-27;
D O I
10.1016/j.apradiso.2012.07.003
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Cross sections for the formation of Ac-225,Ac-227, Ra-223,Ra-225, and Th-227 via the proton bombardment of natural thorium targets were measured at a nominal proton energy of 800 MeV. No earlier experimental cross section data for the production of Ra-223,Ra-225, Ac-227 and Th-227 by this method were found in the literature. A comparison of theoretical predictions with the experimental data shows agreement within a factor of two. Results indicate that accelerator-based production of Ac-225 and Ra-223 is a viable production method. Published by Elsevier Ltd.
引用
收藏
页码:2590 / 2595
页数:6
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