Quantum-dot/organic semiconductor composites for radiation detection

被引:92
作者
Campbell, IH [1 ]
Crone, BK [1 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
关键词
D O I
10.1002/adma.200501434
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A new class of radiation-detection materials, composites of inorganic semiconductor quantum dots and organic semiconductors, that possess the cost and processing advantages of organic scintillators, was described. The composite detector materials were fabricated from CdSe-ZnSe core-shell qdots surface-passivated with hexadecylamine (HDA). The nanoscale mixture of organic and inorganic components should allow the energy from proton recoils off the organic matrix converted to charge by the inorganic semiconductor qdots. The results show that composite materials have processing characteristics similar to organic molecules and polymers and are promising for low-cost, large-area/volume applications.
引用
收藏
页码:77 / 79
页数:3
相关论文
共 10 条
[1]  
Borsenberger PM., 1998, ORGANIC PHOTORECEPTO
[2]   Direct carrier multiplication due to inverse Auger scattering in CdSe quantum dots [J].
Califano, M ;
Zunger, A ;
Franceschetti, A .
APPLIED PHYSICS LETTERS, 2004, 84 (13) :2409-2411
[3]  
Dai S, 2002, AIP CONF PROC, V632, P220
[4]   YIELD OF SINGLET AND TRIPLET EXCITONS FROM X-RAY AND RUBY-LASER EXCITATION OF ANTHRACENE SINGLE-CRYSTALS [J].
HUGHES, RC ;
SOOS, ZG .
JOURNAL OF CHEMICAL PHYSICS, 1975, 63 (03) :1122-1126
[5]   Controlling the morphology of nanocrystal-polymer composites for solar cells [J].
Huynh, WU ;
Dittmer, JJ ;
Libby, WC ;
Whiting, GL ;
Alivisatos, AP .
ADVANCED FUNCTIONAL MATERIALS, 2003, 13 (01) :73-79
[6]  
Knoll GF., 2000, Radiation Detection and Measurement, Vthird
[7]   Photoconductivity in CdSe quantum dot solids [J].
Leatherdale, CA ;
Kagan, CR ;
Morgan, NY ;
Empedocles, SA ;
Kastner, MA ;
Bawendi, MG .
PHYSICAL REVIEW B, 2000, 62 (04) :2669-2680
[8]  
Pope M., 1999, ELECT PROCESSES ORGA
[9]   High efficiency carrier multiplication in PbSe nanocrystals: Implications for solar energy conversion [J].
Schaller, RD ;
Klimov, VI .
PHYSICAL REVIEW LETTERS, 2004, 92 (18) :186601-1
[10]   Quantum dots tailored with poly(para-phenylene vinylene) [J].
Skaff, H ;
Sill, K ;
Emrick, T .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2004, 126 (36) :11322-11325