Source apportionment of fine particles in Kuwait City

被引:78
作者
Alolayan, Mohammad A. [1 ]
Brown, Kathleen W. [2 ]
Evans, John S. [2 ]
Bouhamra, Walid S. [3 ,4 ]
Koutralds, Petros [2 ]
机构
[1] Kuwait Univ, Coll Women, Dept Environm Technol Management, Safat 13060, Kuwait
[2] Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Exposure Epidemiol & Risk Program, Boston, MA 02115 USA
[3] Cyprus Int Inst Environm & Publ Hlth, CY-3041 Limassol, Cyprus
[4] Kuwait Univ, Coll Engn & Petr, Safat 13060, Kuwait
关键词
Apportionment; Emission; Kuwait; PM2.5; PMF; Trajectory; PARTICULATE MATTER; DAILY MORTALITY; AIR-POLLUTION; SAHARAN DUST; IDENTIFICATION; ASSOCIATION; AEROSOLS; SYSTEM; PM2.5; PM10;
D O I
10.1016/j.scitotenv.2012.11.090
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study investigated major sources of PM2.5 in the atmosphere of Kuwait based on a sampling program conducted between February 2004 and October 2005. Three source identification techniques were used in this study: (I) a positive matrix factorization model; (2) backward trajectory profiles; and (3) concentration rose plots. Five major sources of PM2.5 were estimated. These were sand dust (sand storms), oil combustion (power plants), petrochemical industry (fertilizer, nylon or catalyst regeneration facilities), traffic (vehicle emissions and road dust) and transported emissions (emissions from outside Kuwait, such as those from automobiles, road dust or smelters). The estimated contributions to PM2.5 of these sources were: 54% from sand dust, 18% from oil combustion, 12% from petrochemical industry, 11% from traffic and 5% from anthropogenic sources transported from outside the country. Oil combustion, petrochemical industry and traffic were found to emanate from local sources, whereas sand dust and some emissions from traffic, and possibly smelters, appeared to originate from sources outside of Kuwait (transported). The PM2.5 levels in Kuwait during our previous sampling study averaged 53 mu g/m(3). More than half of the measured PM2.5 appears to have been due to crustal material, much originating outside of the country. However, the relatively high levels of PM2.5 contributed by anthropogenic local sources, such as oil combustion, petrochemical industry emissions, and traffic indicated that there may be great opportunities for Kuwait to improve public health. The application of cost-effective emission controls and development of forward looking environmental health policies have the potential to significantly reduce emissions, population exposures to PM2.5 and the burden of mortality and morbidity from air pollution. (C) 2012 Elsevier B.V. All rights reserved.
引用
收藏
页码:14 / 25
页数:12
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