Planar Chirality and Optical Spin-Orbit Coupling for Chiral Fabry-Perot Cavities

被引:30
|
作者
Gautier, Jerome [1 ]
Li, Minghao [1 ]
Ebbesen, Thomas W. [1 ]
Genet, Cyriaque [1 ]
机构
[1] Univ Strasbourg, CNRS, Inst Sci & Ingn Supramol, UMR 7006, F-67000 Strasbourg, France
基金
欧洲研究理事会;
关键词
optical spin-orbit interaction; chirality; circular dichroism; tansfer-matrix; optical cavity; EXCITONS; FIELD;
D O I
10.1021/acsphotonics.1c00780
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
We design, in a most simple way, Fabry-Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin-orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry.
引用
收藏
页码:778 / 783
页数:6
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