Thousand-fold Enhancement of Single-Molecule Fluorescence Near a Single Gold Nanorod

被引：168
作者：
Yuan, Haifeng [1 ]
Khatua, Saumyakanti [1 ]
Zijlstra, Peter [2 ]
Yorulmaz, Mustafa [1 ]
Orrit, Michel [1 ]
机构：
[1] Leiden Univ, MoNOS, Huygens Lab, NL-2300 RA Leiden, Netherlands
[2] Eindhoven Univ Technol, Dept Appl Phys, NL-5600 MB Eindhoven, Netherlands
来源：
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 04期
基金：
欧洲研究理事会;
关键词：
enhanced fluorescence; fluorescence correlation spectroscopy; gold nanorods; single molecules; surface plasmons; CORRELATION SPECTROSCOPY; QUANTUM YIELD; MICROSCOPY; EMISSION; NANOANTENNA;
D O I：
10.1002/anie.201208125
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Single molecules: Large enhancements of single-molecule fluorescence up to 1100 times by using synthesized gold nanorods are reported (see picture). This high enhancement is achieved by selecting a dye with its adsorption and emission close to the surface plasmon resonance of the gold nanorods. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码：1217 / 1221
页数：5
相关论文
共 32 条
  • [1] ALTERATIONS OF SINGLE-MOLECULE FLUORESCENCE LIFETIMES IN NEAR-FIELD OPTICAL MICROSCOPY
    AMBROSE, WP
    GOODWIN, PM
    MARTIN, JC
    KELLER, RA
    [J]. SCIENCE, 1994, 265 (5170) : 364 - 367
  • [2] Enhancement and quenching of single-molecule fluorescence
    Anger, P
    Bharadwaj, P
    Novotny, L
    [J]. PHYSICAL REVIEW LETTERS, 2006, 96 (11)
  • [3] [Anonymous], 2005, ANGEW CHEM INT EDIT, V44, P560
  • [4] Nanoscale spectroscopy with optical antennas
    Bharadwaj, Palash
    Beams, Ryan
    Novotny, Lukas
    [J]. CHEMICAL SCIENCE, 2011, 2 (01) : 136 - 140
  • [5] HIGH-PRESSURE STUDIES OF EFFECT OF VISCOSITY ON FLUORESCENCE EFFICIENCY IN CRYSTAL VIOLET AND AURAMINE O
    BREY, LA
    SCHUSTER, GB
    DRICKAMER, HG
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1977, 67 (06) : 2648 - 2650
  • [6] Unidirectional Emission of a Quantum Dot Coupled to a Nanoantenna
    Curto, Alberto G.
    Volpe, Giorgio
    Taminiau, Tim H.
    Kreuzer, Mark P.
    Quidant, Romain
    van Hulst, Niek F.
    [J]. SCIENCE, 2010, 329 (5994) : 930 - 933
  • [7] Plasmon Emission Quantum Yield of Single Gold Nanorods as a Function of Aspect Ratio
    Fang, Ying
    Chang, Wei-Shun
    Willingham, Britain
    Swanglap, Pattanawit
    Dominguez-Medina, Sergio
    Link, Stephan
    [J]. ACS NANO, 2012, 6 (08) : 7177 - 7184
  • [8] Single quantum dot coupled to a scanning optical antenna: A tunable superemitter
    Farahani, JN
    Pohl, DW
    Eisler, HJ
    Hecht, B
    [J]. PHYSICAL REVIEW LETTERS, 2005, 95 (01)
  • [9] Plasmon-Enhanced Fluorescence from Single Fluorophores End-Linked to Gold Nanorods
    Fu, Yi
    Zhang, Jian
    Lakowicz, Joseph R.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (16) : 5540 - +
  • [10] Detection limits in photothermal microscopy
    Gaiduk, Alexander
    Ruijgrok, Paul V.
    Yorulmaz, Mustafa
    Orrit, Michel
    [J]. CHEMICAL SCIENCE, 2010, 1 (03) : 343 - 350
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