Spatially and spectrally resolved quantum path interference with chirped driving pulses

被引:28
作者
Carlstrom, Stefanos [1 ]
Preclikova, Jana [1 ,2 ]
Lorek, Eleonora [1 ]
Larsen, Esben Witting [1 ]
Heyl, Christoph M. [1 ]
Palecek, David [3 ,4 ]
Zigmantas, Donatas [3 ]
Schafer, Kenneth J. [5 ]
Gaarde, Mette B. [5 ]
Mauritsson, Johan [1 ]
机构
[1] Lund Univ, Dept Phys, Box 118, SE-22210 Lund, Sweden
[2] Univ Bergen, Dept Phys & Technol, N-5007 Bergen, Norway
[3] Lund Univ, Dept Chem Phys, Box 124, SE-22210 Lund, Sweden
[4] Charles Univ Prague, Dept Chem Phys, Ke Karlovu 3, Prague 12116 2, Czech Republic
[5] Louisiana State Univ, Baton Rouge, LA 70803 USA
基金
瑞典研究理事会;
关键词
high-order harmonic generation; quantum path interference; dipole phase parameters; ORDER HARMONIC-GENERATION; ATTOSECOND PULSES; TEMPORAL COHERENCE; FREQUENCY CHIRP; LASER FIELDS; RARE-GASES; RADIATION; IONIZATION; PHASE;
D O I
10.1088/1367-2630/aa511f
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The structures are of two kinds; off-axis interference from the long trajectory only and on-axis interference including the short and long trajectories. The former is readily visible in the far-field spectrum, modulating both the spectral and spatial profile. To access the latter, we vary the chirp of the fundamental, imparting different phases on the different trajectories, thereby changing their relative phase. Using this method together with an analytical model, we are able to explain the on-axis behaviour and access the dipole phase parameters for the short (alpha(s)) and long (alpha(l)) trajectories. The extracted results compare very well with phase parameters calculated by solving the time-dependent Schrodinger equation. Going beyond the analytical model, we are also able to successfully reproduce the off-axis interference structure.
引用
收藏
页数:17
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