Circular dichroism in K-shell ionization from fixed-in-space CO and N2 molecules -: art. no. 073002

被引:124
作者
Jahnke, T
Weber, T
Landers, AL
Knapp, A
Schössler, S
Nickles, J
Kammer, S
Jagutzki, O
Schmidt, L
Czasch, A
Osipov, T
Arenholz, E
Young, AT
Muiño, RD
Rolles, D
de Abajo, FJG
Fadley, CS
Van Hove, MA
Semenov, SK
Cherepkov, NA
Rösch, J
Prior, MH
Schmidt-Böcking, H
Cocke, CL
Dörner, R
机构
[1] Univ Frankfurt, Inst Kernphys, D-60486 Frankfurt, Germany
[2] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA
[3] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA
[4] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA
[5] Donostia Int Phys Ctr, San Sebastian 20018, Spain
[6] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA
[7] State Univ Aerosp Instrumentat, St Petersburg 190000, Russia
关键词
D O I
10.1103/PhysRevLett.88.073002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We have measured the angular distributions of 1s photoelectrons excited by circularly and linearly polarized light from fixed-in-space CO and N-2 molecules, in the vicinity of their shape resonances. A strong circular dichroism, i.e., a strong dependence on the sense of rotation of the polarization vector of the photons, is found for both molecules. State-of-the-art one-electron multiple scattering and partially correlated random phase approximation calculations are in good agreement with many, but not all, aspects of the experimental data.
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页数:4
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共 19 条
[1]   Manifestation of many-electron correlations in photoionization of the K shell of N2 [J].
Cherepkov, NA ;
Semenov, SK ;
Hikosaka, Y ;
Ito, K ;
Motoki, S ;
Yagishita, A .
PHYSICAL REVIEW LETTERS, 2000, 84 (02) :250-253
[2]   CIRCULAR-DICHROISM OF MOLECULES IN THE CONTINUOUS ABSORPTION REGION [J].
CHEREPKOV, NA .
CHEMICAL PHYSICS LETTERS, 1982, 87 (04) :344-348
[3]   Cold Target Recoil Ion Momentum Spectroscopy:: a 'momentum microscope' to view atomic collision dynamics [J].
Dörner, R ;
Mergel, V ;
Jagutzki, O ;
Spielberger, L ;
Ullrich, J ;
Moshammer, R ;
Schmidt-Böcking, H .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 2000, 330 (2-3) :95-192
[4]   CIRCULAR-DICHROISM IN PHOTOELECTRON ANGULAR-DISTRIBUTIONS FROM ORIENTED LINEAR-MOLECULES [J].
DUBS, RL ;
DIXIT, SN ;
MCKOY, V .
PHYSICAL REVIEW LETTERS, 1985, 54 (12) :1249-1251
[5]   Demonstration of strong forward-backward asymmetry in the C1s photoelectron angular distribution from oriented CO molecules [J].
Heiser, F ;
Gessner, O ;
Viefhaus, J ;
Wieliczek, K ;
Hentges, R ;
Becker, U .
PHYSICAL REVIEW LETTERS, 1997, 79 (13) :2435-2437
[6]   Symmetry-selective observation of the N 1s shape resonance in N2 [J].
Hergenhahn, U ;
Kugeler, O ;
Rüdel, A ;
Rennie, EE ;
Bradshaw, AM .
JOURNAL OF PHYSICAL CHEMISTRY A, 2001, 105 (23) :5704-5708
[7]   CIRCULAR-DICHROISM IN THE ANGULAR-DISTRIBUTION OF CORE PHOTOELECTRONS FROM SI(001) - A PHOTOELECTRON-DIFFRACTION ANALYSIS [J].
KADUWELA, AP ;
XIAO, H ;
THEVUTHASAN, S ;
FADLEY, CS ;
VANHOVE, MA .
PHYSICAL REVIEW B, 1995, 52 (20) :14927-14934
[8]   Photoelectron diffraction mapping:: Molecules illuminated from within -: art. no. 013002 [J].
Landers, A ;
Weber, T ;
Ali, I ;
Cassimi, A ;
Hattass, M ;
Jagutzki, O ;
Nauert, A ;
Osipov, T ;
Staudte, A ;
Prior, MH ;
Schmidt-Böcking, H ;
Cocke, CL ;
Dörner, R .
PHYSICAL REVIEW LETTERS, 2001, 87 (01)
[9]   A 4 pi recoil-ion electron momentum analyzer: A high-resolution ''microscope'' for the investigation of the dynamics of atomic, molecular and nuclear reactions [J].
Moshammer, R ;
Unverzagt, M ;
Schmitt, W ;
Ullrich, J ;
SchmidtBocking, H .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1996, 108 (04) :425-445
[10]   K-shell photoionization of CO: I. Angular distributions of photoelectrons from fixed-in-space molecules [J].
Motoki, S ;
Adachi, J ;
Hikosaka, Y ;
Ito, K ;
Sano, M ;
Soejima, K ;
Yagishita, A ;
Raseev, G ;
Cherepkov, NA .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2000, 33 (20) :4193-4212