Imaging the time-dependent structure of a molecule as it undergoes dynamics -: art. no. 052717

被引:91
作者
Légaré, F
Lee, KF
Litvinyuk, IV
Dooley, PW
Bandrauk, AD
Villeneuve, DM
Corkum, PB
机构
[1] Natl Res Council Canada, Ottawa, ON K1A 0R6, Canada
[2] Univ Sherbrooke, Dept Chim, Sherbrooke, PQ J1K 2R1, Canada
[3] McMaster Univ, Dept Phys & Astron, Hamilton, ON K1S 5P3, Canada
[4] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA
来源
PHYSICAL REVIEW A | 2005年 / 72卷 / 05期
关键词
D O I
10.1103/PhysRevA.72.052717
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We image the dynamics of diatomic and triatomic molecules with sub-5 fs and sub-A resolution using laser Coulomb explosion imaging with 8 fs pulses. We obtain image information by measuring the vector momenta of all atomic ions produced by explosion of a single molecule. We image vibrating D-2(+) and of dissociating SO22+ and SO23+. Images taken at 0 and 60 fs show that the dissociation of SO22+ produces an SO+ rotational wave packet.
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页数:4
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共 16 条
  • [1] [Anonymous], 2003, CRC Handbook of Chemistry and Physics, V84th
  • [2] Coulomb explosion imaging of fragmentation channels following laser-induced double ionization of N2
    Beylerian, C
    Cornaggia, C
    [J]. JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2004, 37 (13) : L259 - L265
  • [3] Asymmetric nuclear motion of the F1s-ionized state in BF3 probed by quadruple-ion-coincidence momentum imaging
    De Fanis, A
    Saito, N
    Machida, M
    Okada, K
    Chiba, H
    Cassimi, A
    Dörner, R
    Koyano, I
    Ueda, K
    [J]. PHYSICAL REVIEW A, 2004, 69 (02) : 4
  • [4] Direct imaging of rotational wave-packet dynamics of diatomic molecules
    Dooley, PW
    Litvinyuk, IV
    Lee, KF
    Rayner, DM
    Spanner, M
    Villeneuve, DM
    Corkum, PB
    [J]. PHYSICAL REVIEW A, 2003, 68 (02): : 12
  • [5] Mapping of coherent and decohering nuclear wave-packet dynamics in D2+ with ultrashort laser pulses -: art. no. 063408
    Feuerstein, B
    Thumm, U
    [J]. PHYSICAL REVIEW A, 2003, 67 (06): : 4
  • [6] Reaction dynamics of three-body dissociations in triatomic molecules from single-photon double ionization studied by a time- and position-sensitive coincidence method
    Hsieh, S
    Eland, JHD
    [J]. JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1997, 30 (20) : 4515 - 4534
  • [7] Direct imaging of transient molecular structures with ultrafast diffraction
    Ihee, H
    Lobastov, VA
    Gomez, UM
    Goodson, BM
    Srinivasan, R
    Ruan, CY
    Zewail, AH
    [J]. SCIENCE, 2001, 291 (5503) : 458 - 462
  • [8] ROLE OF EXCITED ELECTRONIC STATES IN THE INTERACTIONS OF FAST (MEV) MOLECULAR-IONS WITH SOLIDS AND GASES
    KANTER, EP
    COONEY, PJ
    GEMMELL, DS
    GROENEVELD, KO
    PIETSCH, WJ
    RATKOWSKI, AJ
    VAGER, Z
    ZABRANSKY, BJ
    [J]. PHYSICAL REVIEW A, 1979, 20 (03): : 834 - 854
  • [9] Laser Coulomb-explosion imaging of small molecules -: art. no. 013415
    Légaré, F
    Lee, KF
    Litvinyuk, IV
    Dooley, PW
    Wesolowski, SS
    Bunker, PR
    Dombi, P
    Krausz, F
    Bandrauk, AD
    Villeneuve, DM
    Corkum, PB
    [J]. PHYSICAL REVIEW A, 2005, 71 (01):
  • [10] Time-resolved double ionization with few cycle laser pulses -: art. no. 093002
    Légaré, F
    Litvinyuk, IV
    Dooley, PW
    Quéré, F
    Bandrauk, AD
    Villeneuve, DM
    Corkum, PB
    [J]. PHYSICAL REVIEW LETTERS, 2003, 91 (09)