Development of a Cloud-Based Epidermal MoSe2 Device for Hazardous Gas Sensing

被引:157
作者
Guo, Shiqi [1 ]
Yang, Dong [2 ,3 ,4 ]
Zhang, Sheng [4 ]
Dong, Quan [1 ]
Li, Baichen [1 ]
Tran, Nam [1 ]
Li, Zhenyu [1 ]
Xiong, Yujie [2 ,3 ]
Zaghloul, Mona E. [1 ]
机构
[1] George Washington Univ, Sch Engn & Appl Sci, Washington, DC 20052 USA
[2] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, IChEM Collaborat Innovat Ctr Chem Energy Mat, Hefei 230026, Anhui, Peoples R China
[3] Univ Sci & Technol China, Sch Chem & Mat Sci, Hefei 230026, Anhui, Peoples R China
[4] Harvard Med Sch, Div Biomed Engn, Brigham & Womens Hosp, Renal Div,Dept Med, Cambridge, MA 02139 USA
基金
美国国家卫生研究院;
关键词
2D material; cloud data; epidermal electronics; gas sensor; CHEMICAL-VAPOR-DEPOSITION; OXIDE NANOSTRUCTURES; GRAPHENE; MONOLAYER; SENSOR; PHOTODETECTORS; EXFOLIATION; ELECTRONICS; TRANSISTORS; DISULFIDES;
D O I
10.1002/adfm.201900138
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Toxic gases such as NO2 and irritant gases such as NH3 are two of the harshest aspects that trigger the exacerbation of the respiratory system for asthma patients. Monitoring and recording high-risk gases are very important for tracking disease and alerting patients because humans can be exposed to a vulnerable environment with inconspicuous gases. Current detectors suffer from lack of portability and cannot provide daily real-time detection. This work develops a light, inexpensive epidermal gas sensor based on ultralarge MoSe2 nanosheets. MoSe2 nanosheets are obtained using a gold-assisted exfoliation method and the electrical and optical properties of the film are characterized. A high-performance gas sensor for NO2 and NH3, which can be integrated onto human skin, is fabricated and shows great stability with up to 30% tensile strain. In particular, the device is able to detect down to 1 part per million with fast response (<200 s). The system is effective in providing timely warnings and the sensing data are uploaded to a cloud-based terminal so that a medical institute can easily access them and provide a more accurate diagnosis.
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页数:10
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