Metal-organic frameworks derived magneticFe3O4/C for catalytic transfer hydrogenation of furfural to furfuryl alcohol

被引：17

作者：

Jiang, Shanshan ^{[1
]}

Huang, Jin ^{[1
,2
]}

Wang, Yue ^{[1
]}

Lu, Shiyu ^{[1
]}

Li, Pei ^{[1
]}

Li, Cuiqin ^{[1
]}

Li, Feng ^{[1
]}

机构：

[1] Northeast Petr Univ, Coll Chem & Chem Engn, Prov Key Lab Oil & Gas Chem Technol, Daqing 163318, Peoples R China

[2] Daqing Normal Univ, Prov Key Lab Oilfield Appl Chem & Technol, Daqing, Peoples R China

来源：

JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY | 2021年 / 96卷 / 03期

关键词：

furfural; transfer hydrogenation; Fe3O4; metal organic frameworks; MEERWEIN-PONNDORF-VERLEY; LITHIUM-ION BATTERIES; SELECTIVE HYDROGENATION; ANODE MATERIALS; EFFICIENT; DEGRADATION; NANOCOMPOSITES; 2-METHYLFURAN; MICROSPHERES; COMPOSITES;

D O I：

10.1002/jctb.6577

中图分类号：

Q81 [生物工程学（生物技术）]; Q93 [微生物学];

学科分类号：

071005 ; 0836 ; 090102 ; 100705 ;

摘要：

AbstactBACKGROUND Fe based metal organic frameworks (Fe-MOFs) were prepared by solvothermal method, and carbon loaded Fe3O4(Fe3O4/C) was prepared by pyrolytic carbonization and carbothermal reduction. RESULTS Various analytical techniques were used to characterize the physicochemical structure of Fe-MOFs and Fe3O4/C under different solvothermal and calcination conditions. Fe3O4/C was then employed as a catalyst for the catalytic transfer hydrogenation of furfural with alcohol as a hydrogen donor, and the effect of hydrogen donor species, reaction temperature, and reaction time were investigated. CONCLUSION The Fe3O4/C catalyst could be easily collected with a magnet and reused for four runs without significant loss of its catalytic. A possible mechanism for the catalytic transfer hydrogenation of furfural over Fe3O4/C was proposed. (c) 2020 Society of Chemical Industry (SCI)

引用

页码：639 / 649

页数：11

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