Molecular spins for quantum computation

被引:622
作者
Gaita-Arino, A. [1 ]
Luis, F. [2 ]
Hill, S. [3 ,4 ]
Coronado, E. [1 ]
机构
[1] Univ Valencia, Inst Ciencia Mol ICMol, Paterna, Spain
[2] Univ Zaragoza, CSIC, Inst Ciencia Mat Aragon, Zaragoza, Spain
[3] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA
[4] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA
关键词
SINGLE-ION MAGNETS; ATOMIC CLOCK; READ-OUT; DESIGN; QUBITS; INFORMATION; COMPLEXES; COHERENCE; OSCILLATIONS; DECOHERENCE;
D O I
10.1038/s41557-019-0232-y
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Spins in solids or in molecules possess discrete energy levels, and the associated quantum states can be tuned and coherently manipulated by means of external electromagnetic fields. Spins therefore provide one of the simplest platforms to encode a quantum bit (qubit), the elementary unit of future quantum computers. Performing any useful computation demands much more than realizing a robust qubit-one also needs a large number of qubits and a reliable manner with which to integrate them into a complex circuitry that can store and process information and implement quantum algorithms. This 'scalability' is arguably one of the challenges for which a chemistry-based bottom-up approach is best-suited. Molecules, being much more versatile than atoms, and yet microscopic, are the quantum objects with the highest capacity to form non-trivial ordered states at the nanoscale and to be replicated in large numbers using chemical tools.
引用
收藏
页码:301 / 309
页数:9
相关论文
共 84 条
  • [1] Heterodimetallic [LnLn′] Lanthanide Complexes: Toward a Chemical Design of Two-Qubit Molecular Spin Quantum Gates
    Aguila, David
    Barrios, Leoni A.
    Velasco, Veronica
    Roubeau, Olivier
    Repolles, Ana
    Alonso, Pablo J.
    Sese, Javier
    Teat, Simon J.
    Luis, Fernando
    Aromi, Guillem
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (40) : 14215 - 14222
  • [2] Synthesis and Properties of a Family of Unsymmetric Dinuclear Complexes of LnIII (Ln = Eu, Gd, Tb)
    Aguila, David
    Barrios, Leoni A.
    Luis, Fernando
    Repolles, Ana
    Roubeau, Olivier
    Teat, Simon J.
    Aromi, Guillem
    [J]. INORGANIC CHEMISTRY, 2010, 49 (15) : 6784 - 6786
  • [3] Mononuclear lanthanide single-molecule magnets based on polyoxometalates
    AlDamen, Murad A.
    Clemente-Juan, Juan M.
    Coronado, Eugenio
    Marti-Gastaldo, Carlos
    Gaita-Arino, Alejandro
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (28) : 8874 - +
  • [4] Mononuclear Lanthanide Single Molecule Magnets Based on the Polyoxometalates [Ln(W5O18)2]9- and [Ln(β2-SiW11O39)2]13- (LnIII = Tb, Dy, Ho, Er, Tm, and Yb)
    AlDamen, Murad A.
    Cardona-Serra, Salvador
    Clemente-Juan, Juan M.
    Coronado, Eugenio
    Gaita-Arino, Alejandro
    Marti-Gastaldo, Carlos
    Luis, Fernando
    Montero, Oscar
    [J]. INORGANIC CHEMISTRY, 2009, 48 (08) : 3467 - 3479
  • [5] Engineering coherent interactions in molecular nanomagnet dimers
    Ardavan, Arzhang
    Bowen, Alice M.
    Fernandez, Antonio
    Fielding, Alistair J.
    Kaminski, Danielle
    Moro, Fabrizio
    Muryn, Christopher A.
    Wise, Matthew D.
    Ruggi, Albert
    McInnes, Eric J. L.
    Severin, Kay
    Timco, Grigore A.
    Timmel, Christiane R.
    Tuna, Floriana
    Whitehead, George F. S.
    Winpenny, Richard E. P.
    [J]. NPJ QUANTUM INFORMATION, 2015, 1
  • [6] Will spin-relaxation times in molecular magnets permit quantum information processing?
    Ardavan, Arzhang
    Rival, Olivier
    Morton, John J. L.
    Blundell, Stephen J.
    Tyryshkin, Alexei M.
    Timco, Grigore A.
    Winpenny, Richard E. P.
    [J]. PHYSICAL REVIEW LETTERS, 2007, 98 (05)
  • [7] Design of magnetic coordination complexes for quantum computing
    Aromi, Guillem
    Aguila, David
    Gamez, Patrick
    Luis, Fernando
    Roubeau, Olivier
    [J]. CHEMICAL SOCIETY REVIEWS, 2012, 41 (02) : 537 - 546
  • [8] A two-qubit molecular architecture for electron-mediated nuclear quantum simulation
    Atzori, Matteo
    Chiesa, Alessandro
    Morra, Elena
    Chiesa, Mario
    Sorace, Lorenzo
    Carretta, Stefano
    Sessoli, Roberta
    [J]. CHEMICAL SCIENCE, 2018, 9 (29) : 6183 - 6192
  • [9] Room-Temperature Quantum Coherence and Rabi Oscillations in Vanadyl Phthalocyanine: Toward Multifunctional Molecular Spin Qubits
    Atzori, Matteo
    Tesi, Lorenzo
    Morra, Elena
    Chiesa, Mario
    Sorace, Lorenzo
    Sessoli, Roberta
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2016, 138 (07) : 2154 - 2157
  • [10] Room temperature quantum coherence in a potential molecular qubit
    Bader, Katharina
    Dengler, Dominik
    Lenz, Samuel
    Endeward, Burkhard
    Jiang, Shang-Da
    Neugebauer, Petr
    van Slageren, Joris
    [J]. NATURE COMMUNICATIONS, 2014, 5