Photoelectron angular distributions for the two-photon ionization of helium by ultrashort extreme ultraviolet free-electron laser pulses

被引:20
作者
Ma, R. [1 ,2 ,3 ]
Motomura, K. [1 ,2 ]
Ishikawa, K. L. [4 ]
Mondal, S. [1 ]
Fukuzawa, H. [1 ,2 ]
Yamada, A. [1 ,2 ]
Ueda, K. [1 ,2 ]
Nagaya, K. [2 ,5 ]
Yase, S. [2 ,5 ]
Mizoguchi, Y. [2 ,5 ]
Yao, M. [2 ]
Rouze, A. [6 ,7 ]
Hundermark, A. [6 ,7 ]
Vrakking, M. J. J. [6 ,7 ]
Johnsson, P. [8 ]
Nagasono, M. [2 ]
Tono, K. [9 ]
Togashi, T. [9 ]
Senba, Y. [9 ]
Ohashi, H. [2 ,9 ]
Yabashi, M. [2 ]
Ishikawa, T. [2 ]
机构
[1] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[2] RIKEN SPring 8 Ctr, Mikazuki, Hyogo 6795148, Japan
[3] Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Peoples R China
[4] Univ Tokyo, Photon Sci Ctr, Grad Sch Engn, Bunkyo Ku, Tokyo 1138656, Japan
[5] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan
[6] Max Born Inst, D-12489 Berlin, Germany
[7] FOM Inst AMOLF, NL-1098 XG Amsterdam, Netherlands
[8] Lund Univ, Dept Phys, SE-22100 Lund, Sweden
[9] Japan Synchrotron Radiat Res Inst, Sayo, Hyogo 6795198, Japan
基金
瑞典研究理事会;
关键词
ABOVE-THRESHOLD IONIZATION; SINGLE IONIZATION; FEMTOSECOND; COHERENCE; OPERATION; ATOMS; PHASE; HE;
D O I
10.1088/0953-4075/46/16/164018
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The two-photon ionization of helium atoms by ultrashort extreme-ultraviolet free-electron laser pulses, produced by the SPring-8 Compact SASE Source test accelerator, was investigated at photon energies of 20.3, 21.3, 23.0 and 24.3 eV. The angular distribution of photoelectrons generated by two-photon ionization is obtained using a velocity map imaging spectrometer. The phase-shift differences and amplitude ratios of the outgoing s and d continuum wave packets are extracted from the photoelectron angular distributions. The obtained values of the phase-shift differences are distinct from scattering phase-shift differences when the photon energy is tuned to a resonance with an excited level or Rydberg manifold. The difference stems from the co-presence of resonant and non-resonant path contributions in the two-photon ionization by femtosecond pulses. Since the relative contribution of both paths can be controlled in principle by the pulse shape, these results illustrate a new way to tailor the continuum wave packet.
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页数:6
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