Low-temperature spin excitations in frustrated ZnCr2O4 probed by high-field thermal conductivity

被引:10
作者
Zhou, H. D. [1 ,2 ]
Zhao, Z. Y. [3 ]
Sun, X. F. [3 ]
Nieto Suarez, M. [4 ]
Rivas-Murias, B. [4 ]
Tsurkan, V. [5 ,6 ]
Deisenhofer, J. [5 ]
Zapf, V. S. [7 ]
Rivadulla, F. [4 ]
机构
[1] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[2] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA
[3] Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
[4] Ctr Invest Quim Biol & Mat Mol CIQUS, Santiago De Compostela 15782, Spain
[5] Univ Augsburg, Ctr Elect Correlat & Magnetism, D-86159 Augsburg, Germany
[6] Moldavian Acad Sci, Inst Appl Phys, MD-2028 Kishinev, Moldova
[7] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA
来源
PHYSICAL REVIEW B | 2013年 / 87卷 / 17期
基金
中国国家自然科学基金;
关键词
RESONATING VALENCE BONDS; SUPERCONDUCTIVITY; ICE;
D O I
10.1103/PhysRevB.87.174436
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The magnetoelastic excitations of spin frustrated ZnCr2O4 are studied by the magnetic field dependence of the thermal conductivity k down to 50 mK. Above the first-order magnetostructural transition at T-N,T-S approximate to 12.5 K, spin fluctuations are strongly coupled to acoustic phonons, leading to a glasslike dependence of k(T), up to Theta(CW). In the symmetry broken phase below T-N,T-S, k shows a dominant magnetic contribution even at the lowest temperatures probed in this work. Application of a magnetic field above 2.5 T destabilizes the spin-bond structure, leading to a sudden increase and a nonconventional temperature dependence of the thermal conductivity. The possibility of the coexistence of gapped and gapless excitations in this magnetic phase is discussed.
引用
收藏
页数:4
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