Progress in the determination of the sea spray source function using satellite data

被引:6
作者
Albert, Monique F. M. A. [1 ]
Schaap, Martijn [1 ]
de Leeuw, Gerrit [1 ,2 ,3 ]
Builtjes, Peter J. H. [1 ]
机构
[1] TNO, Business Unit Environm Hlth & Safety, Utrecht, Netherlands
[2] Finnish Meteorol Inst, Climate Change Unit, FIN-00101 Helsinki, Finland
[3] Univ Helsinki, Dept Phys, Helsinki, Finland
关键词
marine aerosol; remote sensing; climate;
D O I
10.1080/19438151003621466
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Sea spray aerosol influences climate considerably through both direct and indirect aerosol effects. Climate models contain a sea spray source function, i.e. the emission rate of sea spray aerosol droplets per unit area of the sea surface, currently parameterised in terms of wind speed and sea surface temperature (SST). The uncertainty between different formulations of the sea spray source function, and thus associated with the calculated emission fluxes for sea spray aerosol, is more than a factor of 2. In addition, the fraction of organic material in sub-micrometer sea spray droplets is highly uncertain. It is expected that improved estimates can be obtained by inclusion of factors, such as wave conditions, whitecap fraction, improved SST, salinity, and chlorophyll concentration. We aim to incorporate these factors in a new sea spray emission model constrained by the use of satellite observations. Here, we present a methodology for estimating the global primary marine sub-micron organic matter emission. As a first estimate we found an annual global emission of about 20 TgC.
引用
收藏
页码:159 / 166
页数:8
相关论文
共 24 条
[1]   THE SPRAY CONTRIBUTION TO NET EVAPORATION FROM THE SEA - A REVIEW OF RECENT PROGRESS [J].
ANDREAS, EL ;
EDSON, JB ;
MONAHAN, EC ;
ROUAULT, MP ;
SMITH, SD .
BOUNDARY-LAYER METEOROLOGY, 1995, 72 (1-2) :3-52
[2]   Whitecap coverage from satellite measurements: A first step toward modeling the variability of oceanic whitecaps [J].
Anguelova, MD ;
Webster, F .
JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS, 2006, 111 (C3)
[3]  
[Anonymous], 2004, Sea salt aerosol production: mechanisms, methods, measurements and models: a critical review
[4]   Assessment of uncertainty in the ocean reflectance determined by three satellite ocean color sensors (MERIS, SeaWiFS and MODIS-A) at an offshore site in the Mediterranean Sea (BOUSSOLE project) [J].
Antoine, David ;
d'Ortenzio, Fabrizio ;
Hooker, Stanford B. ;
Becu, Guislain ;
Gentili, Bernard ;
Tailliez, Dominique ;
Scott, Alec J. .
JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS, 2008, 113 (C7)
[5]   Advances in characterization of size-resolved organic matter in marine aerosol over the North Atlantic [J].
Cavalli, F ;
Facchini, MC ;
Decesari, S ;
Mircea, M ;
Emblico, L ;
Fuzzi, S ;
Ceburnis, D ;
Yoon, YJ ;
O'Dowd, CD ;
Putaud, JP ;
Dell'Acqua, A .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D24) :1-14
[6]   Primary submicron marine aerosol dominated by insoluble organic colloids and aggregates [J].
Facchini, Maria Cristina ;
Rinaldi, Matteo ;
Decesari, Stefano ;
Carbone, Claudio ;
Finessi, Emanuela ;
Mircea, Mihaela ;
Fuzzi, Sandro ;
Ceburnis, Darius ;
Flanagan, Robert ;
Nilsson, E. Douglas ;
de Leeuw, Gerrit ;
Martino, Manuela ;
Woeltjen, Janina ;
O'Dowd, Colin D. .
GEOPHYSICAL RESEARCH LETTERS, 2008, 35 (17)
[7]   A new physically-based quantification of marine isoprene and primary organic aerosol emissions [J].
Gantt, B. ;
Meskhidze, N. ;
Kamykowski, D. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (14) :4915-4927
[8]   A parameterization of sea-salt aerosol source function for sub- and super-micron particles [J].
Gong, SL .
GLOBAL BIOGEOCHEMICAL CYCLES, 2003, 17 (04)
[9]  
Hu C, 2007, ENV S 2007 MONTR SWI
[10]   New Directions: Organic matter contribution to marine aerosols and cloud condensation nuclei [J].
Langmann, Baerbel ;
Scannell, Claire ;
O'Dowd, Colin .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (33) :7821-7822