Monolithic, microchannel and carbon nanofibers/carbon felt reactors for syngas conversion by Fischer-Tropsch synthesis

被引:49
作者
Holmen, Anders [1 ]
Venvik, Hilde J. [1 ]
Myrstad, Rune [2 ]
Zhu, Jun [1 ]
Chen, De [1 ]
机构
[1] Norwegian Univ Sci & Technol NTNU, Dept Chem Engn, N-7491 Trondheim, Norway
[2] SINTEF Mat & Chem, N-7465 Trondheim, Norway
关键词
Syngas conversion; Fischer-Tropsch; Cobalt; Microchannel reactors; Monoliths; Carbon felt; SUPPORTED COBALT CATALYSTS; HIGH THERMAL-CONDUCTIVITY; PARTICLE-SIZE; HYDROCARBON SELECTIVITY; PARTIAL OXIDATION; SURFACE OXYGEN; METHANE; SSITKA;
D O I
10.1016/j.cattod.2013.06.006
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The present contribution summarizes work carried out on different microstructured reactors in the Catalysis Group at the Norwegian University of Science and Technology during the last years. The work has involved co-operation with industry (Statoil) as well as foreign groups (University of Karlsruhe). The experimental work covers monolithic reactors made of different materials, microchannel reactors and some recent work using carbon nanofibers/carbon felt (CNF/CF). The summary is focused on syngas conversion by the Fischer-Tropsch synthesis, but references to work on methanol and DME production in microreactors are also included. Supported Co-based catalysts are used for the Fischer-Tropsch synthesis and the results are compared with experiments carried out in a standard fixed-bed reactor using the same type of catalysts. A monolithic/microreactor/catalyst concept for Fischer-Tropsch synthesis offers several possible advantages compared to other Fischer-Tropsch reactors and could be of interest for offshore installations and distributed small scale production. (C) 2013 Elsevier B.V. All rights reserved.
引用
收藏
页码:150 / 157
页数:8
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