Nonadiabatic theory of strong-field atomic effects under elliptical polarization

被引:19
作者
Wang, Xu [1 ]
Eberly, J. H.
机构
[1] Univ Rochester, Rochester Theory Ctr, Rochester, NY 14627 USA
关键词
DOUBLE-IONIZATION; MULTIPHOTON IONIZATION; HARMONIC-GENERATION; MOLECULES; DYNAMICS; PHYSICS; HELIUM;
D O I
10.1063/1.4752079
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Elliptically polarized laser fields provide a new channel for access to strong-field processes that are either suppressed or not present under linear polarization. Quantum theory is mostly unavailable for their analysis, and we report here results of a systematic study based on a classical ensemble theory with solution of the relevant ab inito time-dependent Newton equations for selected model atoms. The study's approach is necessarily nonadiabatic, as it follows individual electron trajectories leading to single, double, and triple ionizations. Of particular interest are new results bearing on open questions concerning experimental reports of unexplained species dependences as well as double-electron release times that are badly matched by a conventional adiabatic quantum tunneling theory. We also report the first analysis of electron trajectories for sequential and non-sequential triple ionization. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4752079]
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页数:9
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