Mass transfer in a rotating packed bed reactor with a mesh-pin rotor: Modeling and experimental studies

被引:39
作者
Liu, Wei [1 ,2 ]
Chu, Guang-Wen [1 ,2 ]
Luo, Yong [1 ,2 ]
Liu, Ya-Zhao [1 ,2 ]
Meng, Fan-Yong [3 ]
Sun, Bao-Chang [1 ,2 ]
Chen, Jian-Feng [1 ,2 ]
机构
[1] Beijing Univ Chem Technol, Minist Educ High Grav Engn & Technol, Res Ctr, Beijing 100029, Peoples R China
[2] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
[3] Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
基金
中国国家自然科学基金;
关键词
Rotating packed bed reactor; Mesh-pin rotor; Mass transfer; Model; Liquid holdup; CATALYTIC OXIDATIVE ABSORPTION; HYDROGEN-SULFIDE; LIQUID HOLDUP; FLOW; REMOVAL; GAS; PACKING;
D O I
10.1016/j.cej.2019.03.081
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A rotating packed bed (RPB) reactor with full stainless steel wire mesh packing loaded in the rotor has excellent mass transfer performance. However, it has the blockage problem when applied to the reactions with solid generated on the surface of the packing. In this work, a mesh-pin rotor (MPR), combining an inner wire mesh packing zone (IMZ) and an outer resin pin zone (OPZ), was designed with the purpose of anti-blockage for the first time, expecting to possess the high mass transfer performance of wire mesh packing and self-cleaning performance of cylindrical pins. With the assistance of liquid holdup measurement by X-Ray CT scan technology, a mass transfer model was proposed for the RPB reactor with MPR and the liquid-side volumetric mass transfer coefficient (k(L)a(e)) was measured by using an oxygen-water desorption system. The predicted results by the model showed good agreement with the experimental results within a deviation of +/- 20%, displaying potential application prospects.
引用
收藏
页码:600 / 610
页数:11
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