Life cycle assessment and costing of urine source separation: Focus on nonsteroidal anti-inflammatory drug removal

被引:61
作者
Landry, Kelly A. [1 ]
Boyer, Treavor H. [2 ]
机构
[1] Univ Florida, Engn Sch Sustainable Infrastruct & Environm, Dept Environm Engn Sci, POB 116450, Gainesville, FL 32611 USA
[2] Arizona State Univ, Sch Sustainable Engn & Built Environm, POB 873005, Tempe, AZ 85287 USA
基金
美国国家科学基金会;
关键词
Life cycle assessment; Life cycle costing; Urine source separation; Nonsteroidal anti-inflammatory drugs; Ion-exchange; Wastewater treatment; WASTE-WATER TREATMENT; PERSONAL CARE PRODUCTS; TREATMENT PLANTS; PHARMACEUTICAL CONCENTRATIONS; STRUVITE PRECIPITATION; ENVIRONMENTAL IMPACTS; NUTRIENT MANAGEMENT; MUSK FRAGRANCES; MICROPOLLUTANTS; EFFICIENCY;
D O I
10.1016/j.watres.2016.09.024
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Urine source separation has the potential to reduce pharmaceutical loading to the environment, while enhancing nutrient recovery. The focus of this life cycle assessment (LCA) was to evaluate the environmental impacts and economic costs to manage nonsteroidal anti-inflammatory drugs (NSAIDs) (i.e., diclofenac, ibuprofen, ketoprofen and naproxen) and nutrients in human urine. Urine source separation was compared with centralized wastewater treatment (WWT) (biological or upgraded with ozonation). The current treatment method (i.e., centralized biological WWT) was compared with hypothetical treatment scenarios (i.e., centralized biological WWT upgraded with ozonation, and urine source separation). Alternative urine source separation scenarios included varying collection and handling methods (i.e., collection by vacuum truck, vacuum sewer, or decentralized treatment), pharmaceuticals removal by ion-exchange, and struvite precipitation. Urine source separation scenarios had 90% lower environmental impact (based,on the TRACI impact assessment method) compared with the centralized wastewater scenarios due to reduced potable water production for flush water, reduced electricity use at the wastewater treatment plant, and nutrient offsets from struvite precipitation. Despite the greatest reduction of pharmaceutical toxicity, centralized treatment upgraded with ozone had the greatest ecotoxicity impacts due to ozonation, operation and infrastructure. Among urine source separation scenarios, decentralized treatment of urine and centralized treatment of urine collected by vacuum truck had negligible cost differences compared with centralized wastewater treatment. Centralized treatment of urine collected by vacuum sewer and centralized treatment with ozone cost 30% more compared with conventional wastewater treatment. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:487 / 495
页数:9
相关论文
共 72 条
[1]   PPCPs in wastewater - Update and calculation of characterization factors for their inclusion in LCA studies [J].
Alfonsin, C. ;
Hospido, A. ;
Omil, F. ;
Moreira, M. T. ;
Feijoo, G. .
JOURNAL OF CLEANER PRODUCTION, 2014, 83 :245-255
[2]   Understanding the removal mechanisms of PPCPs and the influence of main technological parameters in anaerobic UASB and aerobic CAS reactors [J].
Alvarino, T. ;
Suarez, S. ;
Lema, J. M. ;
Omil, F. .
JOURNAL OF HAZARDOUS MATERIALS, 2014, 278 :506-513
[3]  
Andersson J., 2007, RESULTS SWEDISH NATL
[4]  
[Anonymous], 2007, 15 SWISS CTR LIF CYC
[5]  
[Anonymous], TOOL RED ASS CHEM OT
[6]  
[Anonymous], 2010, LIFE CYCLE INVENTORY
[7]  
[Anonymous], 2007, LIFE CYCLE INVENTORI
[8]   Experiences from the implementation of a urine separation system: Goals, planning, reality [J].
Berndtsson, JC .
BUILDING AND ENVIRONMENT, 2006, 41 (04) :427-437
[9]   Evaluating the degradation, sorption, and negative mass balances of pharmaceuticals and personal care products during wastewater treatment [J].
Blair, Benjamin ;
Nikolaus, Adam ;
Hedman, Curtis ;
Klaper, Rebecca ;
Grundl, Timothy .
CHEMOSPHERE, 2015, 134 :395-401
[10]   Determination of the solid-water distribution coefficient (Kd) for pharmaceuticals, estrogens and musk fragrances in digested sludge [J].
Carballa, Marta ;
Fink, Guido ;
Omil, Francisco ;
Lema, Juan M. ;
Ternes, Thomas .
WATER RESEARCH, 2008, 42 (1-2) :287-295