Vibration and two-photon absorption

被引：76

作者：

Bishop, DM ^{[1
]}

Luis, JM

Kirtman, B

机构：

[1] Univ Ottawa, Dept Chem, Ottawa, ON K1N 6N5, Canada

[2] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA

[3] Univ Girona, Dept Chem, Girona 17071, Catalonia, Spain

[4] Univ Girona, Inst Computat Chem, Girona 17071, Catalonia, Spain

来源：

JOURNAL OF CHEMICAL PHYSICS | 2002年 / 116卷 / 22期

关键词：

D O I：

10.1063/1.1477179

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A treatment of nuclear vibrational motions in two-photon absorption is laid out in detail. Perturbation theory is used to develop working formulas for diatomic molecules and tested for the X (1)Sigma(+)-A (1)Pi transition of carbon monoxide. The results are compared with the exact numerical values. Certain vibrational contributions, not previously recognized, are found to make an important contribution to the two-photon absorption probability. (C) 2002 American Institute of Physics.

引用

页码：9729 / 9739

页数：11

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