One-Pot Three-Component Synthesis of Vicinal Diamines via In Situ Aminal Formation and Carboamination

被引:42
作者
Orcel, Ugo [1 ]
Waser, Jerome [1 ]
机构
[1] Ecole Polytech Fed Lausanne, ISIC, LCSO, SB, BCH 4306, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会;
关键词
alkenes; aminals; homogeneous catalysis; Pd catalysis; vicinal diamines; CATALYZED ALKENE CARBOAMINATION; COPE-TYPE HYDROAMINATION; MANNICH-TYPE REACTION; OXIDATIVE CYCLIZATION; ASYMMETRIC-SYNTHESIS; ALLYLIC AMINES; CHIRAL AMIDALS; DIRECT ACCESS; DIAMINATION; PALLADIUM;
D O I
10.1002/anie.201607318
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A synthesis of vicinal diamines via in situ aminal formation and carboamination of allyl amines is reported. Employing highly electron-poor trifluoromethyl aldimines in their stable hemiaminal form was key to enable both a fast and complete aminal formation as well as the palladium-catalyzed carboamination step. The conditions developed allow the introduction of a wide variety of alkynyl, vinyl, aryl, and hetereoaryl groups with complete regioselectivity and high diastereoselectivity. The reaction exhibits a high functional-group tolerance. Importantly, either nitrogen atom of the imidazolidine products can be selectively deprotected, while removal of the aminal tether can be achieved in a single step under mild conditions to reveal the free diamine. We expect that this work will promote the further use of mixed aminal tethers in organic synthesis.
引用
收藏
页码:12881 / 12885
页数:5
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