Rhodium(III)-Catalyzed Enantiotopic C-HActivation Enables Access to P-Chiral Cyclic Phosphinamides

被引:181
作者
Sun, Yang [1 ]
Cramer, Nicolai [1 ]
机构
[1] EPFL SB ISIC LCSA, Lab Asymmetr Catalysis & Synth, BCH 4305, CH-1015 Lausanne, Switzerland
基金
欧洲研究理事会; 瑞士国家科学基金会;
关键词
asymmetric catalysis; C-H activation; chiral Cp ligands; P-chirality; rhodium; H BOND ACTIVATION; STEREOGENIC PHOSPHORUS-COMPOUNDS; ASYMMETRIC-SYNTHESIS; CYCLOPENTADIENYL LIGANDS; ENANTIOSELECTIVE SYNTHESIS; QUATERNARY STEREOCENTERS; DIRECTING GROUPS; BIARYL COMPOUNDS; METAL CATALYSIS; BRONSTED ACID;
D O I
10.1002/anie.201606637
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Compounds with stereogenic phosphorus atoms are frequently used as ligands for transition-metal as well as organocatalysts. A direct catalytic enantioselective method for the synthesis of P-chiral compounds from easily accessible diaryl phosphinamides is presented. The use of rhodium(III) complexes equipped with a suitable atropochiral cyclopentadienyl ligand is shown to enable an enantiodetermining C-H activation step. Upon trapping with alkynes, a broad variety of cyclic phosphinamides with a stereogenic phosphorus(V) atom are formed in high yields and enantioselectivities. Moreover, these can be reduced enantiospecifically to P-chiral phosphorus(III) compounds.
引用
收藏
页码:364 / 367
页数:4
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