The function of zeolite on Pt autoreduction and dispersion in Pt/L and Pt/beta catalysts

被引:12
作者
Zheng, J [1 ]
Dong, JL [1 ]
Xu, QH [1 ]
Hu, C [1 ]
机构
[1] NANJING UNIV,SOLID STATE MICROSTRUCT LAB,NANJING 210093,PEOPLES R CHINA
关键词
autoreduction; dispersion of Pt; L and P zeolites; n-hexane aromatization;
D O I
10.1007/BF00813514
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
TPR, CO-FTIR and Xe-129 NMR spectroscopic techniques were used to measure the distribution of platinum species after the calcination of Pt/L and Pt/beta zeolites. Autoreduction which occurred in Pt/beta zeolite was avoided in the channel of L zeolite. Pt particles dispersed well and exhibited excellent reactivity for the aromatization of n-hexane in L zeolite.
引用
收藏
页码:25 / 28
页数:4
相关论文
共 12 条
[1]  
BERNARD JR, 1980, 5TH P INT C ZEOL NAP, P686
[2]   A NONPOROUS SUPPORTED-PLATINUM CATALYST FOR AROMATIZATION OF N-HEXANE [J].
DAVIS, RJ ;
DEROUANE, EG .
NATURE, 1991, 349 (6307) :313-315
[3]   NUCLEAR MAGNETIC-RESONANCE STUDY OF XENON ADSORBED ON METAL-NAY ZEOLITES - A NEW METHOD FOR THE DETERMINATION OF THE MEAN NUMBER OF ATOMS IN SMALL METALLIC PARTICLES SUPPORTED ON Y-ZEOLITES [J].
DEMENORVAL, LC ;
FRAISSARD, JP ;
ITO, T .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1982, 78 :403-410
[4]  
DEROUANE EG, 1988, APPL CATAL, V45, P419
[5]  
Hughes T.R., 1986, Stud. Surf. Sci. Catal., V28, P725
[6]  
IGLESIA E, 1993, 10TH P INT C CAT BUD, P993
[7]   AROMATIZATION OF NORMAL-HEXANE BY PLATINUM-CONTAINING MOLECULAR-SIEVES .2. NORMAL-HEXANE REACTIVITY [J].
MIELCZARSKI, E ;
HONG, SB ;
DAVIS, RJ ;
DAVIS, ME .
JOURNAL OF CATALYSIS, 1992, 134 (01) :359-369
[8]   ZEOLITE-SUPPORTED TRANSITION-METAL CATALYSTS BY DESIGN [J].
SACHTLER, WMH .
CATALYSIS TODAY, 1992, 15 (3-4) :419-429
[9]  
TAUSTER SJ, 1988, MATERIALS RES SOC S, V111, P419
[10]   XE-129 NMR PROOF FOR THE DISTRIBUTION OF PLATINUM SPECIES DURING PT/NAY PREPARATION BY H2PTCL6 IMPREGNATION AND PT(NH-3)4(2+) CATION-EXCHANGE METHODS [J].
YANG, OB ;
WOO, SI ;
RYOO, R .
JOURNAL OF CATALYSIS, 1990, 123 (02) :375-382