Hybrid Energy Cell for Degradation of Methyl Orange by Self-Powered Electrocatalytic Oxidation

被引:135
作者
Yang, Ya [1 ]
Zhang, Hulin [1 ]
Lee, Sangmin [1 ]
Kim, Dongseob [3 ]
Hwang, Woonbong [3 ]
Wang, Zhong Lin [1 ,2 ]
机构
[1] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
[2] Chinese Acad Sci, Beijing Inst Nanoenergy & Nanosyst, Beijing, Peoples R China
[3] Pohang Univ Sci & Technol, Dept Mech Engn, Pohang 790784, Gyungbuk, South Korea
基金
新加坡国家研究基金会;
关键词
Hybrid energy cell; triboelectric nanogenerator; pyroelectric nanogenerator; self-powered; methyl orange; electrodegradation; ELECTROCHEMICAL OXIDATION; PYROELECTRIC NANOGENERATORS; PHOTOCATALYTIC DEGRADATION; WASTE-WATER; NANOWIRE;
D O I
10.1021/nl3046188
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In general, methyl orange (MO) can be degraded by an electrocatalytic oxidation process driven by a power source due to the generation of superoxidative hydroxyl radical on the anode. Here, we report a hybrid energy cell that is used for a self-powered electrocatalytic process for the degradation of MO without using an external power source. The hybrid energy cell can simultaneously or individually harvest mechanical and thermal energies. The mechanical energy was harvested by the triboelectric nanogenerator (TENG) fabricated at the top by using a flexible polydimethysiloxane (PDMS) nanowire array with diameters of about 200 nm. A pyroelectric nanogenerator (PENG) was fabricated below the TENG to harvest thermal energy. The power output of the device can be directly used for electrodegradation of MO, demonstrating a self-powered electrocatalytic oxidation process.
引用
收藏
页码:803 / 808
页数:6
相关论文
共 27 条
  • [1] [Anonymous], NANO LETT
  • [2] Direct-Write Piezoelectric Polymeric Nanogenerator with High Energy Conversion Efficiency
    Chang, Chieh
    Tran, Van H.
    Wang, Junbo
    Fuh, Yiin-Kuen
    Lin, Liwei
    [J]. NANO LETTERS, 2010, 10 (02) : 726 - 731
  • [3] 1.6 V Nanogenerator for Mechanical Energy Harvesting Using PZT Nanofibers
    Chen, Xi
    Xu, Shiyou
    Yao, Nan
    Shi, Yong
    [J]. NANO LETTERS, 2010, 10 (06) : 2133 - 2137
  • [4] INDIRECT OXIDATION EFFECT IN ELECTROCHEMICAL OXIDATION TREATMENT OF LANDFILL LEACHATE
    CHIANG, LC
    CHANG, JE
    WEN, TC
    [J]. WATER RESEARCH, 1995, 29 (02) : 671 - 678
  • [5] Cross J.A., 1987, ELECTROSTATICS PRINC
  • [6] DECOLOURIZATION OF DYE-CONTAINING SOLUTIONS BY ELECTROCOAGULATION
    DO, JS
    CHEN, ML
    [J]. JOURNAL OF APPLIED ELECTROCHEMISTRY, 1994, 24 (08) : 785 - 790
  • [7] Flexible triboelectric generator!
    Fan, Feng-Ru
    Tian, Zhong-Qun
    Wang, Zhong Lin
    [J]. NANO ENERGY, 2012, 1 (02) : 328 - 334
  • [8] Hybrid Nanogenerator for Concurrently Harvesting Biomechanical and Biochemical Energy
    Hansen, Benjamin J.
    Liu, Ying
    Yang, Rusen
    Wang, Zhong Lin
    [J]. ACS NANO, 2010, 4 (07) : 3647 - 3652
  • [9] Controlled Growth of Semiconducting Nanowire, Nanowall, and Hybrid Nanostructures on Graphene for Piezoelectric Nanogenerators
    Kumar, Brijesh
    Lee, Keun Young
    Park, Hyun-Kyu
    Chae, Seung Jin
    Lee, Young Hee
    Kim, Sang-Woo
    [J]. ACS NANO, 2011, 5 (05) : 4197 - 4204
  • [10] Pyroelectricity: From ancient curiosity to modern imaging tool
    Lang, SB
    [J]. PHYSICS TODAY, 2005, 58 (08) : 31 - 36