Hydrogen Production From Partial Oxidation of Methane Using an AC Rotating Gliding Arc Reactor

被引:26
作者
Li, Xiao Dong [1 ]
Zhang, Hao [1 ]
Yan, Shi Xin [1 ]
Yan, Jian Hua [1 ]
Du, Chang Ming [2 ]
机构
[1] Zhejiang Univ, Inst Thermal Power Engn, Hangzhou 310027, Zhejiang, Peoples R China
[2] Sun Yat Sen Univ, Sch Environm Sci & Engn, Guangzhou 510275, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
Hydrogen; methane; partial oxidation; plasma; rotating gliding arc (RGA); CORONA DISCHARGE; CONVERSION; PLASMA; GAS; DECOMPOSITION; HYDROCARBONS; AIR;
D O I
10.1109/TPS.2012.2226608
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Hydrogen, as well as petrochemical feedstock, can be produced by the partial oxidation of methane in an alternating-current rotating-gliding-arc plasma driven by swirling flow. The effects of the air ratio (0.6 to 1.6), height of outer cover (25 and 45 cm), supply voltage (6.6 to 11.1 kV), and gas flow rate (6 to 18 L/min) on methane reforming have been investigated. The conversion of methane grows with rising air ratio, whereas hydrogen selectivity first augments and then declines. A higher outer cover was beneficial, and maximum methane conversion attains 80.73%. Higher voltage improves the reactor performance. As gas flow rate grows, both methane conversion and hydrogen selectivity diminish, while power consumption first drops to a minimum value of 8.23 kJ/L H-2 for a flow rate of 16 L/min and then again amplifies.
引用
收藏
页码:126 / 132
页数:7
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