Fabrication of Au-Pd nanoparticles/graphene oxide and their excellent catalytic performance

被引:30
作者
He, Yongqiang [1 ]
Zhang, Nana [2 ]
Zhang, Lei [2 ]
Gong, Qiaojuan [1 ]
Yi, Maocong [2 ]
Wang, Wei [3 ]
Qiu, Haixia [2 ]
Gao, Jianping [2 ]
机构
[1] Yuncheng Univ, Dept Appl Chem, Yuncheng 044000, Peoples R China
[2] Tianjin Univ, Sch Sci, Tianjin 300072, Peoples R China
[3] Tianjin Univ, Sch Chem Engn, Tianjin 300072, Peoples R China
基金
美国国家科学基金会;
关键词
Composites; Nanostructures; Chemical synthesis; Electron microscopy; COUPLING REACTIONS; GRAPHENE OXIDE; FACILE SYNTHESIS; SUZUKI-MIYAURA; ARYL CHLORIDES; REDUCTION; EFFICIENT; OXIDATION;
D O I
10.1016/j.materresbull.2013.12.043
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A simple method to fabricate clean Au-Pd nanoparticles on graphene oxide (Au-Pd NPs/GO) without using any reducing agent or surfactant has been developed. GO simultaneously reduced the Au and Pd precursors to form a stable suspension of the Au-Pd NPs/GO. The nanoparticles were characterized by transmission electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy and inductively coupled plasma. The Au-Pd NPs/GO exhibited catalytic activity for the reduction of 4-nitrophenol to 4-aminophenol and for the Suzuki-Miyaura coupling reaction of chlorobenzene and phenylboronic acid in aqueous media. (C) 2013. Elsevier Ltd. All rights reserved.
引用
收藏
页码:397 / 401
页数:5
相关论文
共 25 条
[1]   General catalysts for the Suzuki-Miyaura and Sonogashira coupling reactions of aryl chlorides and for the coupling of challenging substrate combinations in water [J].
Anderson, KW ;
Buchwald, SL .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2005, 44 (38) :6173-6177
[2]   In situ growth of FeNi alloy nanoflowers on reduced graphene oxide nanosheets and their magnetic properties [J].
Bai, Song ;
Shen, Xiaoping ;
Zhu, Guoxing ;
Xu, Zheng ;
Yang, Juan .
CRYSTENGCOMM, 2012, 14 (04) :1432-1438
[3]   Structural characterization study of FeCo alloy nanoparticles in a highly porous aerogel silica matrix [J].
Carta, D. ;
Mountjoy, G. ;
Gass, M. ;
Navarra, G. ;
Casula, M. F. ;
Corrias, A. .
JOURNAL OF CHEMICAL PHYSICS, 2007, 127 (20)
[4]   Synthesis of "Clean" and Well-Dispersive Pd Nanoparticles with Excellent Electrocatalytic Property on Graphene Oxide [J].
Chen, Xiaomei ;
Wu, Genghuang ;
Chen, Jinmei ;
Chen, Xi ;
Xie, Zhaoxiong ;
Wang, Xiaoru .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (11) :3693-3695
[5]   Improved kinetics of ethanol oxidation on Pd catalysts supported on tungsten carbides/carbon nanotubes [J].
Hu, Fengping ;
Cui, Guofeng ;
Wei, Zidong ;
Shen, Pei Kang .
ELECTROCHEMISTRY COMMUNICATIONS, 2008, 10 (09) :1303-1306
[6]   PREPARATION OF GRAPHITIC OXIDE [J].
HUMMERS, WS ;
OFFEMAN, RE .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1958, 80 (06) :1339-1339
[7]   Efficient and highly selective iron-catalyzed reduction of nitroarenes [J].
Jagadeesh, Rajenahally V. ;
Wienhoefer, Gerrit ;
Westerhaus, Felix A. ;
Surkus, Annette-Enrica ;
Pohl, Marga-Martina ;
Junge, Henrik ;
Junge, Kathrin ;
Beller, Matthias .
CHEMICAL COMMUNICATIONS, 2011, 47 (39) :10972-10974
[8]  
Karthika P, 2012, ADV SCI LETT, V6, P141
[9]   Evidence for atomically dispersed Pd in catalysts supported on carbon nanofibers [J].
Kochubey, D. I. ;
Chesnokov, V. V. ;
Malykhin, S. E. .
CARBON, 2012, 50 (08) :2782-2787
[10]   Reduction of 4-nitrophenol to 4-aminophenol over Au nanoparticles deposited on PMMA [J].
Kuroda, Kyoko ;
Ishida, Tamao ;
Haruta, Masatake .
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2009, 298 (1-2) :7-11