On the current distribution at the channel - rib scale in polymer-electrolyte fuel cells

被引:14
作者
Belgacem, Najib [1 ]
Pauchet, Joel [2 ]
Prat, Marc [1 ]
机构
[1] Univ Toulouse, CNRS, IMFT, INPT,UPS, Toulouse, France
[2] Univ Grenoble Alpes, CEA LITEN, DEHT, 17 Rue Martyrs, F-38054 Grenoble, France
关键词
Current density distribution; Pore network modelling; Condensation; Gas diffusion layer; Rib-channel; Continuum - PNM coupled model; GAS-DIFFUSION LAYERS; PORE-NETWORK; LIQUID WATER; 2-PHASE FLOW; TRANSPORT PHENOMENA; COUPLED CONTINUUM; CATHODE; MODEL; PEFCS; DURABILITY;
D O I
10.1016/j.ijhydene.2018.01.097
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Experimental results based on in-situ measurements at the interface between the catalyst layer and the gas diffusion layer (GDL) on the cathode side at the channel - rib scale show an interesting variation of the current density distribution as the mean current density is increased. It is found that the local current density below the rib median axis corresponds to a maximum at low to intermediate mean current densities and to a minimum when the mean current density is sufficiently high. Also, the higher is the current density, the more marked the minimum. From numerical simulations, it is shown that the current density distribution inversion phenomenon is strongly correlated to the liquid water zone development within the GDL. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:5112 / 5123
页数:12
相关论文
共 39 条
  • [1] Simulation of a Full Fuel Cell Membrane Electrode Assembly Using Pore Network Modeling
    Aghighi, Mahmoudreza
    Hoeh, Michael A.
    Lehnert, Werner
    Merle, Geraldine
    Gostick, Jeff
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2016, 163 (05) : F384 - F392
  • [2] [Anonymous], THESIS
  • [3] Two-phase flow and thermal transients in proton exchange membrane fuel cells - A critical review
    Banerjee, Rupak
    Kandlikar, Satish G.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2015, 40 (10) : 3990 - 4010
  • [4] Coupled continuum and condensation-evaporation pore network model of the cathode in polymer-electrolyte fuel cell
    Belgacem, Najib
    Prat, Marc
    Pauchet, Joel
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (12) : 8150 - 8165
  • [5] Three-dimensional computational analysis of transport phenomena in a PEM fuel cell - a parametric study
    Berning, T
    Djilali, N
    [J]. JOURNAL OF POWER SOURCES, 2003, 124 (02) : 440 - 452
  • [6] A quantitative study of the effect of flow-distributor geometry in the cathode of a PEM fuel cell
    Birgersson, E
    Vynnycky, M
    [J]. JOURNAL OF POWER SOURCES, 2006, 153 (01) : 76 - 88
  • [7] Synchrotron X-ray Radiography as a Highly Precise and Accurate Method for Measuring the Spatial Distribution of Liquid Water in Operating Polymer Electrolyte Membrane Fuel Cells
    Chevalier, S.
    Ge, N.
    George, M. G.
    Lee, J.
    Banerjee, R.
    Liu, H.
    Shrestha, P.
    Muirhead, D.
    Hinebaugh, J.
    Tabuchi, Y.
    Kotaka, T.
    Bazylak, A.
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2017, 164 (02) : F107 - F114
  • [8] A review on water balance in the membrane electrode assembly of proton exchange membrane fuel cells
    Dai, Wei
    Wang, Haijiang
    Yuan, Xiao-Zi
    Martin, Jonathan J.
    Yang, Daijun
    Qiao, Jinli
    Ma, Jianxin
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (23) : 9461 - 9478
  • [9] Durability and degradation issues of PEM fuel cell components
    de Bruijn, F. A.
    Dam, V. A. T.
    Janssen, G. J. M.
    [J]. FUEL CELLS, 2008, 8 (01) : 3 - 22
  • [10] Operando Properties of Gas Diffusion Layers: Saturation and Liquid Permeability
    Eller, Jens
    Roth, Jorg
    Marone, Federica
    Stampanoni, Marco
    Buchi, Felix N.
    [J]. JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2017, 164 (02) : F115 - F126