Constructing a Spatially Resolved Methane Emission Inventory for the Barnett Shale Region

被引:118
作者
Lyon, David R. [1 ,2 ]
Zavala-Araiza, Daniel [1 ]
Alvarez, Ramon A. [1 ]
Harriss, Robert [1 ]
Palacios, Virginia [1 ]
Lan, Xin [3 ]
Talbot, Robert [3 ]
Lavoie, Tegan [4 ]
Shepson, Paul [4 ]
Yacovitch, Tara I. [5 ]
Herndon, Scott C. [5 ]
Marchese, Anthony J. [6 ]
Zimmerle, Daniel [6 ]
Robinson, Allen L. [7 ]
Hamburg, Steven P. [1 ]
机构
[1] Environm Def Fund, Austin, TX 78701 USA
[2] Univ Arkansas, Environm Dynam Program, Fayetteville, AR 72701 USA
[3] Univ Houston, Dept Earth & Atmospher Sci, Houston, TX 77004 USA
[4] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA
[5] Aerodyne Res Inc, Billerica, MA 01821 USA
[6] Colorado State Univ, Dept Mech Engn, Ft Collins, CO 80523 USA
[7] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA
关键词
NATURAL-GAS PRODUCTION; HYDROCARBON EMISSIONS; OIL;
D O I
10.1021/es506359c
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Methane emissions from the oil and gas industry (O&G) and other sources in the Barnett Shale region were estimated by constructing a spatially resolved emission inventory. Eighteen source categories were estimated using multiple data sets, including new empirical measurements at regional O&G sites and a national study of gathering and processing facilities. Spatially referenced activity data were compiled from federal and state databases and combined with O&G facility emission factors calculated using Monte Carlo simulations that account for high emission sites representing the very upper portion, or fat-tail, in the observed emissions distributions. Total methane emissions in the 25-county Barnett Shale region in October 2013 were estimated to be 72,300 (63,400-82,400) kg CH4 h(-1). O&G emissions were estimated to be 46,200 (40,000-54,100) kg CH4 h(-1) with 19% of emissions from fat tail sites representing less than 2% of sites. Our estimate of O&G emissions in the Barnett Shale region was higher than alternative inventories based on the United States Environmental Protection Agency (EPA) Greenhouse Gas Inventory, EPA Greenhouse Gas Reporting Program, and Emissions Database for Global Atmospheric Research by factors of 1.5, 2.7, and 4.3, respectively. Gathering compressor stations, which accounted for 40% of O&G emissions in our inventory, had the largest difference from emission estimates based on EPA data sources. Our inventory's higher O&G emission estimate was due primarily to its more comprehensive activity factors and inclusion of emissions from fat-tail sites.
引用
收藏
页码:8147 / 8157
页数:11
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