Nonperturbative Interband Response of a Bulk InSb Semiconductor Driven Off Resonantly by Terahertz Electromagnetic Few-Cycle Pulses

被引:78
作者
Junginger, F. [1 ,2 ]
Mayer, B. [1 ,2 ]
Schmidt, C. [1 ,2 ]
Schubert, O. [1 ,2 ,3 ]
Maehrlein, S. [1 ,2 ]
Leitenstorfer, A. [1 ,2 ]
Huber, R. [1 ,2 ,3 ]
Pashkin, A. [1 ,2 ]
机构
[1] Univ Konstanz, Dept Phys, D-78457 Constance, Germany
[2] Univ Konstanz, Ctr Appl Photon, D-78457 Constance, Germany
[3] Univ Regensburg, Dept Phys, D-93053 Regensburg, Germany
关键词
FIELD-RESOLVED DETECTION; GENERATION; TRANSIENTS; AMPLITUDES;
D O I
10.1103/PhysRevLett.109.147403
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Intense multiterahertz pulses are used to study the coherent nonlinear response of bulk InSb by means of field-resolved four-wave mixing spectroscopy. At amplitudes above5 MV/cm the signals show a clear temporal substructure which is unexpected in perturbative nonlinear optics. Simulations based on a model of a two-level quantum system demonstrate that in spite of the strongly off-resonant character of the excitation the high-field few-cycle pulses drive the interband resonances into a nonperturbative regime of Rabi flopping. The rotating wave approximation breaks down in this case and the system reaches a complete population inversion.
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页数:5
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