A Small Molecule Composed of Dithienopyran and Diketopyrrolopyrrole as Versatile Electron Donor Compatible with Both Fullerene and Nonfullerene Electron Acceptors for High Performance Organic Solar Cells

被引：69
|
作者：
Jung, Jae Woong [1 ]
Russell, Thomas P. [2 ]
Jo, Won Ho [1 ]
机构：
[1] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151744, South Korea
[2] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA
来源：
CHEMISTRY OF MATERIALS | 2015年 / 27卷 / 13期
关键词：
HIGH PHOTOVOLTAIC EFFICIENCY; POWER CONVERSION EFFICIENCY; BENZODITHIOPHENE UNIT; V-OC; 10-PERCENT; MORPHOLOGY; POLYMERS;
D O I：
10.1021/acs.chemmater.5b01799
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A new conjugated small molecule composed of dithienopyran and diketopyrrolopyrrole (DTP-DPP) was synthesized. Since DTP-DPP has advantageous optoelectronic properties for photovoltaic applications such as intense and broad light absorption, proper frontier energy levels, high crystallinity, and high hole mobility, the devices fabricated from the blend with PC71BM and P(NDI2OD-T2) exhibit high power conversion efficiencies of 6.88% and 4.82%, respectively. This work demonstrates that DTP-DPP is a versatile electron donor compatible with both fullerene and nonfullerene acceptors for high performance SM-OSCs.
引用
收藏
页码：4865 / 4870
页数：6
相关论文
共 50 条
  • [1] A versatile small molecular electron donor with 2-dimensional conjugation structure for efficient organic solar cells compatible with both fullerene and non-fullerene electron acceptors
    Jung, Jae Woong
    DYES AND PIGMENTS, 2019, 161 : 214 - 220
  • [2] A medium-bandgap small molecule donor compatible with both fullerene and unfused-ring nonfullerene acceptors for efficient organic solar cells
    Chen, Xianjie
    Ding, Xueyan
    Zhang, Qian
    Wang, Di
    Zhan, Lingling
    Lu, Xinhui
    Wu, Feifei
    Xu, Zheng
    Qiu, Huayu
    Chen, Wanzhi
    Li, Chang-Zhi
    JOURNAL OF MATERIALS CHEMISTRY C, 2019, 7 (43) : 13396 - 13401
  • [3] Versatile π-bridges in nonfullerene electron acceptors of organic solar cells
    Feng, Fan
    Wang, Pengchao
    Li, Yonghai
    Bao, Xichang
    MATERIALS CHEMISTRY FRONTIERS, 2023, 7 (18) : 3855 - 3878
  • [4] Non-fullerene small molecule electron acceptors for high-performance organic solar cells
    Hao Lin
    Qiang Wang
    Journal of Energy Chemistry, 2018, 27 (04) : 990 - 1016
  • [5] Non-fullerene small molecule electron acceptors for high-performance organic solar cells
    Lin, Hao
    Wang, Qiang
    JOURNAL OF ENERGY CHEMISTRY, 2018, 27 (04) : 990 - 1016
  • [6] Non-fullerene small molecule electron acceptors for high-performance organic solar cells
    Hao Lin
    Qiang Wang
    Journal of Energy Chemistry , 2018, (04) : 990 - 1016
  • [7] Low-Bandgap Small Molecules as Non-Fullerene Electron Acceptors Composed of Benzothiadiazole and Diketopyrrolopyrrole for All Organic Solar Cells
    Jung, Jae Woong
    Jo, Won Ho
    CHEMISTRY OF MATERIALS, 2015, 27 (17) : 6038 - 6043
  • [8] Small molecule donors based on benzodithiophene and diketopyrrolopyrrole compatible with both fullerene and non-fullerene acceptors
    Huo, Yong
    Zhu, Jingshuai
    Wang, Xiao-Zhen
    Yan, Cenqi
    Chai, Yun-Fei
    Chen, Zi-Zhen
    Zhan, Xiaowei
    Zhang, Hao-Li
    JOURNAL OF MATERIALS CHEMISTRY C, 2018, 6 (22) : 5843 - 5848
  • [9] Medium-Bandgap Small-Molecule Donors Compatible with Both Fullerene and Nonfullerene Acceptors
    Huo, Yong
    Yan, Cenqi
    Kan, Bin
    Liu, Xiao-Fei
    Chen, Li-Chuan
    Hu, Chen-Xia
    Lau, Tsz-Ki
    Lu, Xinhui
    Sun, Chun-Lin
    Shao, Xiangfeng
    Chen, Yongsheng
    Zhan, Xiaowei
    Zhang, Hao-Li
    ACS APPLIED MATERIALS & INTERFACES, 2018, 10 (11) : 9587 - 9594
  • [10] Asymmetric Nonfullerene Small Molecule Acceptors for Organic Solar Cells
    Li, Chao
    Fu, Huiting
    Xia, Tian
    Sun, Yanming
    ADVANCED ENERGY MATERIALS, 2019, 9 (25)
12345