High-harmonic generation in ZnO driven by self-compressed mid-infrared pulses

被引:10
作者
Gholam-Mirzaei, Shima [1 ]
Beetar, John E. [1 ]
Chacon, Alexis [3 ]
Chini, Michael [1 ,2 ]
机构
[1] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA
[2] Univ Cent Florida, Coll Opt & Photon, CREOL, Orlando, FL 32816 USA
[3] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA
关键词
PHASE MODULATION; OPTICAL PULSES; SOLIDS; BULK; INTERFEROMETRY; MOLECULES; DYNAMICS; MEDIA;
D O I
10.1364/JOSAB.35.000A27
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Progress in attosecond science has relied on advancements in few-cycle pulse generation technology and its application to high-order harmonic generation. Traditionally, self-phase modulation in bulk solids has been used for the compression of moderate-energy pulses, additionally exhibiting favorable dispersion properties for mid-infrared (mid-IR) pulses. Here, we use the anomalous dispersion of Y3Al5O12 (YAG) to self-compress many-cycle pulses from a 50 kHz mid-IR OPA down to produce sub-three-cycle 10 mu J pulses and further use them to generate high-order harmonics in a ZnO crystal. In agreement with theoretical predictions, we observe a boost in the harmonic yield by a factor of two, and spectral broadening of above-gap harmonics, compared to longer driving pulses. The enhanced yield results from an increase in the intensity for the self-compressed pulses. (C) 2018 Optical Society of America
引用
收藏
页码:A27 / A31
页数:5
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