Robust signatures in the current-voltage characteristics of DNA molecules oriented between two graphene nanoribbon electrodes

被引:24
作者
Paez, Carlos J. [1 ,2 ]
Schulz, Peter A. [1 ,2 ]
Wilson, Neil R. [3 ]
Roemer, Rudolf A. [3 ,4 ]
机构
[1] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil
[2] Univ Estadual Campinas, Fac Ciencias Aplicadas, BR-13484350 Limeira, SP, Brazil
[3] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England
[4] Univ Warwick, Ctr Comp Sci, Coventry CV4 7AL, W Midlands, England
来源
NEW JOURNAL OF PHYSICS | 2012年 / 14卷
基金
英国工程与自然科学研究理事会; 巴西圣保罗研究基金会;
关键词
CHARGE-TRANSPORT; ELECTRICAL-TRANSPORT; HOLE-TRANSFER; LAMBDA-DNA; CONDUCTIVITY; DEVICES; BINDING;
D O I
10.1088/1367-2630/14/9/093049
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In this work, we numerically calculate the electric current through three kinds of DNA sequences (telomeric, lambda-DNA and p53-DNA) described by different heuristic models. A bias voltage is applied between two zigzag edged graphene contacts attached to the DNA segments, while a gate terminal modulates the conductance of the molecule. Calculation of the current is performed by integrating the transmission function (calculated using the lattice Green's function) over the range of energies allowed by the chemical potentials. We show that a telomeric DNA sequence, when treated as a quantum wire in the fully coherent low-temperature regime, works as an excellent semiconductor. Clear steps are apparent in the current-voltage curves of telomeric sequences and are present independent of length and sequence initialization at the contacts. We also find that the molecule-electrode coupling can drastically influence the magnitude of the current. The difference between telomeric DNA and other DNAs, such as lambda-DNA and DNA for the tumour suppressor p53, is particularly visible in the length dependence of the current.
引用
收藏
页数:17
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