Temperature dependence of the electromagnetic and microwave absorption properties of polyimide/Ti3SiC2 composites in the X band

被引:30
作者
Wang, Hongyu [1 ]
Zhu, Dongmei [1 ]
Zhou, Wancheng [1 ]
Luo, Fa [1 ]
机构
[1] Northwestern Polytech Univ, State Key Lab Solidificat Proc, Xian 710072, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
ABSORBING PROPERTIES; CARBON NANOTUBES; NANOCOMPOSITES; SUPERCAPACITOR; GRAPHENE; POWDERS;
D O I
10.1039/c5ra17758h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Ti3SiC2 particles with an average diameter of 5 mm are added into a polyimide matrix to fabricate electromagnetic microwave absorbing materials. The complex permittivity of the composites increases with the increasing Ti3SiC2 content due to an enhanced interface polarization and conduction loss. The maximum reflection loss value of the polyimide/Ti3SiC2 composite is up to -48.6 dB at 8.5 GHz with a thickness of 2.9 mm and the absorption bandwidth below -10 dB is 3.8 GHz. The complex permittivity shows a remarkable temperature dependent effect in the 8.2-12.4 GHz range, and when the temperature is 400 degrees C, the bandwidth below -10 dB is 2.48 GHz with an optimum thickness of 2.0 mm. The excellent absorption properties of the polyimide/Ti3SiC2 composite mean that it can be used as an attractive candidate for a new type of microwave absorption material at elevated temperature.
引用
收藏
页码:86656 / 86664
页数:9
相关论文
共 33 条
[1]   Electrical conductivity, thermopower, and hall effect of Ti3AIC2, Ti4AIN3, and Ti3SiC2 [J].
Barsoum, MW ;
Yoo, HI ;
Polushina, IK ;
Rud, VY ;
Rud, YV ;
El-Raghy, T .
PHYSICAL REVIEW B, 2000, 62 (15) :10194-10198
[2]   Graphene and MWCNT based bi-functional polymer nanocomposites with enhanced microwave absorption and supercapacitor property [J].
Bhattacharya, Pallab ;
Dhibar, Saptarshi ;
Kundu, Mrinal Kanti ;
Hatui, Goutam ;
Das, Chapal K. .
MATERIALS RESEARCH BULLETIN, 2015, 66 :200-212
[3]   In Situ Synthesis and Characterization of CuFe10Al2O19/MWCNT Nanocomposites for Supercapacitor and Microwave-Absorbing Applications [J].
Bhattacharya, Pallab ;
Das, Chapal K. .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2013, 52 (28) :9594-9606
[4]   The effects of temperature and frequency on the dielectric properties, electromagnetic interference shielding and microwave-absorption of short carbon fiber/silica composites [J].
Cao, Mao-Sheng ;
Song, Wei-Li ;
Hou, Zhi-Ling ;
Wen, Bo ;
Yuan, Jie .
CARBON, 2010, 48 (03) :788-796
[5]   Matching design and mismatching analysis towards radar absorbing coatings based on conducting plate [J].
Cao, MS ;
Qin, RR ;
Qiu, CJ ;
Zhu, J .
MATERIALS & DESIGN, 2003, 24 (05) :391-396
[6]   Electromagnetic interference shielding effectiveness of carbon materials [J].
Chung, DDL .
CARBON, 2001, 39 (02) :279-285
[7]   Dielectric properties of Ti2AlC and Ti2AlN MAX phases:: The conductivity anisotropy [J].
Haddad, Noel ;
Garcia-Caurel, Enric ;
Hultman, Lars ;
Barsoum, Michel W. ;
Hug, Gilles .
JOURNAL OF APPLIED PHYSICS, 2008, 104 (02)
[8]   Effects of milling methods on the dielectric and the mechanical properties of hot-pressed sintered MoSi2/Al2O3 composites [J].
Huang, Zhibin ;
Zhou, Wancheng ;
Tang, Xiufeng ;
Zhu, Jiankun .
JOURNAL OF ALLOYS AND COMPOUNDS, 2011, 509 (05) :1920-1923
[9]   High-efficiency and dynamic stable electromagnetic wave attenuation for La doped bismuth ferrite at elevated temperature and gigahertz frequency [J].
Li, Yong ;
Cao, Mao-sheng ;
Wang, Da-wei ;
Yuan, Jie .
RSC ADVANCES, 2015, 5 (94) :77184-77191
[10]   Microwave dielectric properties of Ti3SiC2 powders synthesized by solid state reaction [J].
Li, Zhimin ;
Wei, Xiaohei ;
Luo, Fa ;
Zhou, Wancheng ;
Hao, Yue .
CERAMICS INTERNATIONAL, 2014, 40 (01) :2545-2549