Numerical modeling on simultaneous removal of mercury and particulate matter within an electrostatic precipitator

被引:19
作者
Feng, Yuxuan [1 ]
Gao, Wenchao [2 ]
Zhou, Mengmeng [2 ]
Luo, Kun [1 ]
Fan, Jianren [1 ]
Zheng, Chenghang [1 ]
Gao, Xiang [1 ]
机构
[1] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Peoples R China
[2] Monash Univ, Dept Chem Engn, ARC Res Hub Computat Particle Technol, Clayton, Vic 3800, Australia
关键词
SORBENT INJECTION; FLUE-GAS; HYBRID FILTER; SEWAGE-SLUDGE; COAL; CAPTURE; CARBON; ADSORPTION; PERFORMANCE; COMBUSTION;
D O I
10.1016/j.apt.2020.01.037
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A computational fluid dynamics (CFD) model coupled with gas-particle mass transfer, electrohydrodynamic (EHD) effect, electric field, particle motion and particle charging is established to advance the understanding of combined particulate matter precipitation and mercury capture within industrial electrostatic precipitators (ESPs). The comparisons between experimental data and numerical results demonstrate that this model can reasonably predict the mercury removal efficiency by powdered sorbent injection (PSI). The mechanism of simultaneous removal of mercury and particulate matter is then discussed in detail by considering the complex interactions among multi-physics. The influences of particle size, mercury concentration, particle injection rate and the EHD effect are investigated. The simulation results indicate that the mercury removal process is primarily controlled by the sorbent particle residence time, surface area and mass transfer rate. Accordingly, reducing the size of sorbent particles (activated carbon) can promote mercury removal efficiency while decreasing the particle collection efficiency. Increasing the initial mercury concentration and adsorbent mass loading also benefit mercury adsorption by influencing the mass transfer rate and the surface area. The EHD effect plays important roles in mercury removal and particle collection by means of altering the flow patterns and particle migration. The two mechanisms of in-flight and wall-bounded mercury adsorption affected by ionic wind are also evaluated and some interesting phenomena are observed. © 2020 The Society of Powder Technology Japan
引用
收藏
页码:1759 / 1770
页数:12
相关论文
共 36 条
[1]  
BIRD RB, 1979, ABSTR PAP AM CHEM S, P35
[2]   Full-scale evaluation of sorbent injection for mercury control on coal-fired power plants [J].
Bustard, J ;
Durham, M ;
Starns, T ;
Lindsey, C ;
Martin, C ;
Schlager, R ;
Baldrey, K .
FUEL PROCESSING TECHNOLOGY, 2004, 85 (6-7) :549-562
[3]  
Chen S., 1996, Prepr. Pap.-Am. Chem. Soc., V1996, P442
[4]  
Clack H.L., 2008, 11 INT C EL PREC CHI, P37
[5]  
Clack H.L., 2012, J AIR WASTE MANAGE, V56, P759
[6]   Mass transfer within electrostatic precipitators: In-flight adsorption of mercury by charged suspended particulates [J].
Clack, Herek L. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (11) :3617-3622
[7]   Numerical Simulation of Simultaneous Electrostatic Precipitation and Trace Gas Adsorption: Electrohydrodynamic Effects [J].
Clack, Herek L. .
FRONTIERS IN ENERGY RESEARCH, 2017, 5
[8]   Mercury Capture within Coal-Fired Power Plant Electrostatic Precipitators: Model Evaluation [J].
Clack, Herek L. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (05) :1460-1466
[9]   Mercury emission control in coal-fired plants:: The role of wet scrubbers [J].
Diaz-Somoano, Mercedes ;
Unterberger, Sven ;
Hein, Klaus R. G. .
FUEL PROCESSING TECHNOLOGY, 2007, 88 (03) :259-263
[10]  
Gorji M. Rahimi, 2019, ONCOPOINT 7 RES SEM