Optical trapping of NaYF4:Er3+,Yb3+ upconverting fluorescent nanoparticles

被引:66
作者
Haro-Gonzalez, P. [1 ]
del Rosal, B. [1 ]
Maestro, L. M. [1 ]
Rodriguez, E. Martin [2 ]
Naccache, R. [2 ]
Capobianco, J. A. [2 ]
Dholakia, K. [3 ]
Garcia Sole, J. [1 ]
Jaque, D. [1 ]
机构
[1] Univ Autonoma Madrid, Dept Fis Mat, Fluorescence Imaging Grp, E-28049 Madrid, Spain
[2] Concordia Univ, Ctr NanoSci Res, Dept Chem & Biochem, Montreal, PQ H4B 1R6, Canada
[3] Univ St Andrews, SUPA, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland
基金
英国工程与自然科学研究理事会; 加拿大自然科学与工程研究理事会;
关键词
UP-CONVERSION; SINGLE; PARTICLES; THERMOPHORESIS; SPECTROSCOPY; MANIPULATION;
D O I
10.1039/c3nr03644h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report on the first experimental observation of stable optical trapping of dielectric NaYF4:Er3+,Yb3+ upconverting fluorescent nanoparticles (similar to 26 nm in diameter) using a continuous wave 980 nm single-beam laser. The laser serves both to optically trap and to excite visible luminescence from the nanoparticles. Sequential loading of individual nanoparticles into the trap is observed from the analysis of the emitted luminescence. We demonstrate that the trapping strength and the number of individual nanoparticles trapped are dictated by both the laser power and nanoparticle density. The possible contribution of thermal effects has been investigated by performing trapping experiment in both heavy water and into distilled water. For the case of heavy water, thermal gradients are negligible and optical forces dominate the trap loading behaviour. The results provide a promising path towards real three dimensional manipulation of single NaYF4:Er3+,Yb3+ nanoparticles for precise fluorescence sensing in biophotonics experiments.
引用
收藏
页码:12192 / 12199
页数:8
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