PM2.5 in an industrial district of Zhengzhou, China: Chemical composition and source apportionment

被引:111
作者
Geng, Ningbo [1 ]
Wang, Jia [1 ]
Xu, Yifei [1 ]
Zhang, Wending [1 ]
Chen, Chun [2 ]
Zhang, Ruiqin [1 ]
机构
[1] Zhengzhou Univ, Dept Chem, Res Inst Environm Sci, Zhengzhou 450001, Peoples R China
[2] Henan Environm Monitoring Ctr, Zhengzhou 450004, Henan, Peoples R China
关键词
PM2.5; Component; Seasonal variation; PMF; Source apportionment; FINE PARTICULATE MATTER; ELEMENTAL COMPOSITION; TRACE-ELEMENTS; ION CHEMISTRY; MASS CLOSURE; PARTICLES; URBAN; AEROSOL; PM10; TRENDS;
D O I
10.1016/j.partic.2012.08.004
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Zhengzhou is a developing city in China, that is heavily polluted by high levels of particulate matter. In this study, fine particulate matter (PM2.5) was collected and analyzed for their chemical composition (soluble ions, elements, elemental carbon (EC) and organic carbon (OC)) in an industrial district of Zhengzhou in 2010. The average concentrations of PM2.5 were 181, 122, 186 and 211 mu g/m(3) for spring, summer, autumn and winter, respectively, with an annual average of I 75 mu g/m(3), far exceeding the PM2.5 regulation of USA National Air Quality Standards (15 mu g/m(3)). The dominant components of PM2.5 in Zhengzhou were secondary ions (sulphate and nitrate) and carbon fractions. Soluble ions, total carbon and elements contributed 41%, 13% and 3% of PM2.5 mass, respectively. Soil dust, secondary aerosol and coal combustion, each contributing about 26%, 24% and 23% of total PM2.5 mass, were the major sources of PM2.5, according to the result of positive matrix factorization analysis. A mixed source of biomass burning, oil combustion and incineration contributed 13% of PM2.5. Fine particulate matter arising from vehicles and industry contributed about 10% and 4% of PM2.5, respectively. (C) 2012 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:99 / 109
页数:11
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