An Amorphous Carbon Nitride Photocatalyst with Greatly Extended Visible-Light-Responsive Range for Photocatalytic Hydrogen Generation

被引:863
作者
Kang, Yuyang [1 ]
Yang, Yongqiang [1 ]
Yin, Li-Chang [1 ]
Kang, Xiangdong [1 ]
Liu, Gang [1 ]
Cheng, Hui-Ming [1 ]
机构
[1] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China
关键词
amorphization; carbon nitride; hydrogen; photocatalysts; visible light; SURFACE SCIENCE; WATER; ABSORPTION; CATALYSTS; DIOXIDE; MELON; UV;
D O I
10.1002/adma.201501939
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Amorphous carbon nitride (ACN) with a bandgap of 1.90 eV shows an order of magnitude higher photocatalytic activity in hydrogen evolution under visible light than partially crystalline graphitic carbon nitride with a bandgap of 2.82 eV. ACN is photocatalytically active under visible light at a wavelength beyond 600 nm. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:4572 / 4577
页数:6
相关论文
共 37 条
[1]   Flame-assisted synthesis of nanoscale, amorphous and crystalline, spherical BiVO4 with visible-light photocatalytic activity [J].
Castillo, Nikola C. ;
Heel, Andre ;
Graule, Thomas ;
Pulgarin, Cesar .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2010, 95 (3-4) :335-347
[2]   Increasing Solar Absorption for Photocatalysis with Black Hydrogenated Titanium Dioxide Nanocrystals [J].
Chen, Xiaobo ;
Liu, Lei ;
Yu, Peter Y. ;
Mao, Samuel S. .
SCIENCE, 2011, 331 (6018) :746-750
[3]   Semiconductor-based Photocatalytic Hydrogen Generation [J].
Chen, Xiaobo ;
Shen, Shaohua ;
Guo, Liejin ;
Mao, Samuel S. .
CHEMICAL REVIEWS, 2010, 110 (11) :6503-6570
[4]   Disordered Co1.28Mn1.71O4 as a Visible-Light-Responsive Photocatalyst for Hydrogen Evolution [J].
Chen, Zu Peng ;
Xing, Jun ;
Jiang, Ha Bo ;
Yang, Hua Gui .
CHEMISTRY-A EUROPEAN JOURNAL, 2013, 19 (13) :4123-4127
[5]   The surface science of titanium dioxide [J].
Diebold, U .
SURFACE SCIENCE REPORTS, 2003, 48 (5-8) :53-229
[6]   Structural Investigation of Graphitic Carbon Nitride via XRD and Neutron Diffraction [J].
Fina, Federica ;
Callear, Samantha K. ;
Carins, George M. ;
Irvine, John T. S. .
CHEMISTRY OF MATERIALS, 2015, 27 (07) :2612-2618
[7]   Template-free synthesis of porous graphitic carbon nitride microspheres for enhanced photocatalytic hydrogen generation with high stability [J].
Gu, Quan ;
Liao, Yusen ;
Yin, Lisha ;
Long, Jinlin ;
Wang, Xuxu ;
Xue, Can .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 165 :503-510
[8]   PHOTOELECTROCATALYTIC REDUCTION OF CARBON-DIOXIDE IN AQUEOUS SUSPENSIONS OF SEMICONDUCTOR POWDERS [J].
INOUE, T ;
FUJISHIMA, A ;
KONISHI, S ;
HONDA, K .
NATURE, 1979, 277 (5698) :637-638
[9]   Visible light-driven efficient overall water splitting using p-type metal-nitride nanowire arrays [J].
Kibria, M. G. ;
Chowdhury, F. A. ;
Zhao, S. ;
AlOtaibi, B. ;
Trudeau, M. L. ;
Guo, H. ;
Mi, Z. .
NATURE COMMUNICATIONS, 2015, 6
[10]   Heterogeneous photocatalyst materials for water splitting [J].
Kudo, Akihiko ;
Miseki, Yugo .
CHEMICAL SOCIETY REVIEWS, 2009, 38 (01) :253-278