High Performance Hydrogen/Bromine Redox Flow Battery for Grid-Scale Energy Storage

被引：163
|
作者：
Cho, Kyu Taek [1 ]
Ridgway, Paul [1 ]
Weber, Adam Z. [1 ]
Haussener, Sophia [1 ,2 ]
Battaglia, Vincent [1 ]
Srinivasan, Venkat [1 ]
机构：
[1] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA
[2] Ecole Polytech Fed Lausanne, Inst Engn Mech, CH-1015 Lausanne, Switzerland
来源：
JOURNAL OF THE ELECTROCHEMICAL SOCIETY | 2012年 / 159卷 / 11期
关键词：
BROMINE; ELECTRODE; CELL; MEMBRANES; ADSORPTION; OXIDATION; ANIONS; MODEL;
D O I：
10.1149/2.018211jes
中图分类号：
O646 [电化学、电解、磁化学];
学科分类号：
081704 ;
摘要：
The electrochemical behavior of a promising hydrogen/bromine redox flow battery is investigated for grid-scale energy-storage application with some of the best redox-flow-battery performance results to date, including a peak power of 1.4 W/cm(2) and a 91% voltaic efficiency at 0.4 W/cm(2) constant-power operation. The kinetics of bromine on various materials is discussed, with both rotating-disk-electrode and cell studies demonstrating that a carbon porous electrode for the bromine reaction can conduct platinum-comparable performance as long as sufficient surface area is realized. The effect of flow-cell designs and operating temperature is examined, and ohmic and mass-transfer losses are decreased by utilizing a flow-through electrode design and increasing cell temperature. Charge/discharge and discharge-rate tests also reveal that this system has highly reversible behavior and good rate capability. (C) 2012 The Electrochemical Society. [DOI: 10.1149/2.018211jes] All rights reserved.
引用
收藏
页码：A1806 / A1815
页数：10
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