Synthesis of nanoclusters and quasy one-dimensional structures in glow discharge atT≈ 2 K

被引:4
作者
Boltnev, R. E. [1 ,2 ,3 ]
Kononov, E. A. [1 ,3 ]
Trukhachev, F. M. [1 ,3 ]
Vasiliev, M. M. [1 ,3 ]
Petrov, O. F. [1 ,3 ]
机构
[1] Russian Acad Sci, Joint Inst High Temp, 13-2 Izhorskaya Str, Moscow 125412, Russia
[2] Russian Acad Sci, Chernogolovka Branch, NN Semenov Fed Res Ctr Chem Phys, Chernogolovka 142432, Moscow Region, Russia
[3] Moscow Inst Phys & Technol, Dolgoprudnyi 141701, Moscow Region, Russia
基金
俄罗斯科学基金会;
关键词
DC glow discharge; ultracold dusty plasma; sputtering; nanoclusters; synthesis; self-assembly; HELIUM PLASMA; DUST; SEMICONDUCTOR; CARBON; CLOUD;
D O I
10.1088/1361-6595/aba2ab
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The present article considers the phenomena observed in ultracold multimodal dusty plasma generated in the glow discharge cooled with superfluid helium. It was shown that intense sputtering of the clay insert due to focused beams of low energy electrons and ions produces a total flow similar to 100 ng s(-1)of sputtered materials at the power released in the discharge less than 0.1 W atT <= 2 K. The synthesis rates for nanoclusters (similar to 10 ng s(-1)) and filaments (similar to 1 ng s(-1)) were estimated for the first time. Fast growth of quasy one-dimensional structures, the filaments with high aspect ratio, similar to 100, in ultracold plasma was explained by self-assembly of polarizable materials in strongly inhomogeneous electric fields. The intense broadband emission stimulated by laser excitation of the filaments synthesized was assigned to carbon quantum dots, domains enriched with carbon. The key parameters of the nanocluster cloud were determined for the first time. The nanocluster concentration was estimated as high as 10(12)divided by 10(13)nanocluster/m(3). Charging of nanoclusters in plasma produced a stable uprising nanocluster flow (similar to 10(8)cluster/s) driven by external electrostatic field and observable due to laser light scattering on dust acoustic waves developed within the flow. Temporal variations of the nanocluster concentration caused changes of the interparticle distance in the dusty plasma structure composed of CeO(2)particles. It was found that the particles trapped in the structure had the mean size of about 2 mu m and much narrower size distribution in comparison with the very broad initial distribution.
引用
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页数:10
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