Magnetic excitation spectrum of Na2IrO3 probed with resonant inelastic x-ray scattering

被引:82
作者
Gretarsson, H. [1 ]
Clancy, J. P. [1 ]
Singh, Yogesh [2 ]
Gegenwart, P. [3 ]
Hill, J. P. [4 ]
Kim, Jungho [5 ]
Upton, M. H. [5 ]
Said, A. H. [5 ]
Casa, D. [5 ]
Gog, T. [5 ]
Kim, Young-June [1 ]
机构
[1] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada
[2] Indian Inst Sci Educ & Res Mohali, Manauli 140306, PO, India
[3] Univ Gottingen, Inst Phys 1, D-37077 Gottingen, Germany
[4] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA
[5] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
基金
加拿大自然科学与工程研究理事会;
关键词
D O I
10.1103/PhysRevB.87.220407
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The low energy excitations in Na2IrO3 have been investigated using resonant inelastic x-ray scattering (RIXS). A magnetic excitation branch can be resolved, whose dispersion reaches a maximum energy of about 35 meV at the Gamma point. The momentum dependence of the excitation energy is much larger along the Gamma-X direction compared to that along the Gamma-Y direction. The observed dispersion relation is consistent with a recent theoretical prediction based on the Heisenberg-Kitaev model. At high temperatures, we find large contributions from lattice vibrational modes to our RIXS spectra, suggesting that a strong electron-lattice coupling is present in Na2IrO3.
引用
收藏
页数:5
相关论文
共 36 条
  • [1] Quantum oscillations of nitrogen atoms in uranium nitride
    Aczel, A. A.
    Granroth, G. E.
    MacDougall, G. J.
    Buyers, W. J. L.
    Abernathy, D. L.
    Samolyuk, G. D.
    Stocks, G. M.
    Nagler, S. E.
    [J]. NATURE COMMUNICATIONS, 2012, 3
  • [2] Determining the electron-phonon coupling strength from Resonant Inelastic X-ray Scattering at transition metal L-edges
    Ament, L. J. P.
    van Veenendaal, M.
    van den Brink, J.
    [J]. EPL, 2011, 95 (02)
  • [3] Resonant inelastic x-ray scattering studies of elementary excitations
    Ament, Luuk J. P.
    van Veenendaal, Michel
    Devereaux, Thomas P.
    Hill, John P.
    van den Brink, Jeroen
    [J]. REVIEWS OF MODERN PHYSICS, 2011, 83 (02) : 705 - 767
  • [4] Spin-orbital locking, emergent pseudo-spin and magnetic order in honeycomb lattice iridates
    Bhattacharjee, Subhro
    Lee, Sung-Sik
    Kim, Yong Baek
    [J]. NEW JOURNAL OF PHYSICS, 2012, 14
  • [5] Magnetic Excitations and Phase Separation in the Underdoped La2-xSrxCuO4 Superconductor Measured by Resonant Inelastic X-Ray Scattering
    Braicovich, L.
    van den Brink, J.
    Bisogni, V.
    Moretti Sala, M.
    Ament, L. J. P.
    Brookes, N. B.
    De Luca, G. M.
    Salluzzo, M.
    Schmitt, T.
    Strocov, V. N.
    Ghiringhelli, G.
    [J]. PHYSICAL REVIEW LETTERS, 2010, 104 (07)
  • [6] Dispersion of Magnetic Excitations in the Cuprate La2CuO4 and CaCuO2 Compounds Measured Using Resonant X-Ray Scattering
    Braicovich, L.
    Ament, L. J. P.
    Bisogni, V.
    Forte, F.
    Aruta, C.
    Balestrino, G.
    Brookes, N. B.
    De Luca, G. M.
    Medaglia, P. G.
    Granozio, F. Miletto
    Radovic, M.
    Salluzzo, M.
    van den Brink, J.
    Ghiringhelli, G.
    [J]. PHYSICAL REVIEW LETTERS, 2009, 102 (16)
  • [7] Chaloupka G, PHYS REV LETT, V105
  • [8] Chaloupka G. Jackeli, PHYS REV LETT, V110
  • [9] Spin Waves and Revised Crystal Structure of Honeycomb Iridate Na2IrO3
    Choi, S. K.
    Coldea, R.
    Kolmogorov, A. N.
    Lancaster, T.
    Mazin, I. I.
    Blundell, S. J.
    Radaelli, P. G.
    Singh, Yogesh
    Gegenwart, P.
    Choi, K. R.
    Cheong, S. -W.
    Baker, P. J.
    Stock, C.
    Taylor, J.
    [J]. PHYSICAL REVIEW LETTERS, 2012, 108 (12)
  • [10] Spin-orbit coupling in iridium-based 5d compounds probed by x-ray absorption spectroscopy
    Clancy, J. P.
    Chen, N.
    Kim, C. Y.
    Chen, W. F.
    Plumb, K. W.
    Jeon, B. C.
    Noh, T. W.
    Kim, Young-June
    [J]. PHYSICAL REVIEW B, 2012, 86 (19)