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3D tree-shaped hierarchical flax fabric for highly efficient solar steam generation
被引:63
|作者:
Li, Yaping
[1
,2
]
Fan, Jie
[1
,2
]
Wang, Run
[2
]
Shou, Wan
[3
]
Wang, Liang
[2
]
Liu, Yong
[2
]
机构:
[1] Tiangong Univ, Key Lab Adv Text Mat, Minist Educ, Tianjin 300387, Peoples R China
[2] Tiangong Univ, Sch Text Sci & Engn, Tianjin 300387, Peoples R China
[3] MIT, Dept Elect Engn & Comp Sci, Comp Sci & Articial Intelligence Lab, Cambridge, MA 02139 USA
基金:
国家重点研发计划;
关键词:
LOW-COST;
WATER;
POLYPYRROLE;
DESALINATION;
NANOPARTICLES;
POLYANILINE;
NANOFIBERS;
CARBON;
D O I:
10.1039/d0ta09570b
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Solar steam generation as a promising technology has great potential for application in wastewater treatment and seawater desalination. However, it remains challenging to develop low-cost, high-efficiency steam generators that are suitable for large scale application. Here, inspired by the natural transpiration process of trees, we fabricated a three-dimensional (3D) hierarchical tree-shaped biomimetic flax fabric (TBFF) using an ordinary loom, consisting of a float layer, basket weave layer and plain weave layer, which showed directional water transport properties along the continuous warp yarns of the fabric. Then, the obtained TBFF was modified by one-step synthesis of large-area polydopamine-polypyrrole composite (PDA-PPy) nanofibers for a high hydrophilicity and a higher surface area. The hierarchical micro-capillary pores of yarns and macro-interlaced pore structures between the warp and weft yarns in such modified TBFF-PDA-PPy exhibit broadband light absorption, high-efficiency water supply, large evaporation area, and easy steam escape. Therefore, the continuous water transport paths formed by TBFF-PDA-PPy could deliver an attractive evaporation rate of 1.37 kg m(-2) h(-1), where the solar energy conversion efficiency was up to 87.4% under 1 sun illumination. Based on the facile fabrication, low cost and scalable manufacturing process, this nature-inspired design of 3D hierarchical TBFF-PDA-PPy is expected to promote large-scale applications in water purification and seawater desalination.
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页码:2248 / 2258
页数:11
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