Photocatalytic degradation of organic dyes with Er3+:YAlO3/ZnO composite under solar light

被引:87
作者
Wang, Jun [1 ,2 ]
Xie, Yingpeng [1 ]
Zhang, Zhaohong [3 ]
Li, Jia [1 ]
Chen, Xia [1 ]
Zhang, Liquan [2 ]
Xu, Rui [1 ]
Zhang, Xiangdong [1 ]
机构
[1] Liaoning Univ, Dept Chem, Shenyang 110036, Peoples R China
[2] Liaoning Univ, Dept Pharm, Shenyang 110036, Peoples R China
[3] Liaoning Univ, Dept Environm, Shenyang 110036, Peoples R China
基金
中国国家自然科学基金;
关键词
Er3+:YAlO3/ZnO composite; Upconversion luminescence agent; Photocatalytic degradation; Solar light; Organic dye; UP-CONVERSION LUMINESCENCE; VISIBLE-LIGHT; AZO-DYE; ZNO; TIO2; IRRADIATION; WATER; SEMICONDUCTOR; CATALYST; PHOTODEGRADATION;
D O I
10.1016/j.solmat.2008.11.017
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The Er3+:YAlO3/ZnO composite, a new photocatalyst that could effectively utilize visible light, was prepared by ultrasonic dispersion and liquids boiling method in this work. In succession, the Er3+:YAlO3/ZnO composite, Er3+:YAlO3 particle and pure ZnO powder were characterized by X-ray diffraction (XRD). The Acid Red B dye as a model compound was degraded under solar light irradiation to evaluate the photocatalytic activity of the Er3+:YAlO3/ZnO composite. In addition, the effects of Er3+:YAlO3 content, heat-treated temperature and heat-treated time on photocatalytic activity of Er3+:YAlO3/ZnO composite were reviewed through the degradation of Acid Red B dye under solar light. Otherwise, the effects of initial concentration, Er3+:YAlO3/ZnO amount, solution acidity and solar light irradiation time on the photocatalytic degradation of Acid Red B dye were investigated in detail. It was found that the photocatalytic activity of Er3+ :YAlO3/ZnO composite is much higher than that of pure ZnO powder for the similar system. Perhaps, the use of this Er3+:YAlO3/ZnO composite may provide a new way to take advantage of ZnO in sewage treatment aspects using solar energy. (C) 2008 Elsevier B.V. All rights reserved.
引用
收藏
页码:355 / 361
页数:7
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