Plasmon Ag nanoparticle/Bi2S3 ultrathin nanobelt/oxygen-doped flower-like MoS2 nanosphere ternary heterojunctions for promoting charge separation and enhancing solar-driven photothermal and photocatalytic performances

被引:101
作者
Jiang, Hao [1 ]
Xing, Zipeng [1 ]
Zhao, Tianyu [1 ]
Yang, Zekang [1 ]
Wang, Ke [1 ]
Li, Zhenzi [3 ]
Yang, Shilin [1 ]
Xie, Luyan [2 ]
Zhou, Wei [1 ,3 ]
机构
[1] Heilongjiang Univ, Sch Chem & Mat Sci, Dept Environm Sci, Key Lab Funct Inorgan Mat Chem,Minist Educ People, Harbin 150080, Peoples R China
[2] Harbin Engn Univ, Harbin 150001, Peoples R China
[3] Qilu Univ Technol, Sch Chem & Pharmaceut Engn, Shandong Prov Key Lab Mol Engn, Shandong Acad Sci, Jinan 250353, Peoples R China
基金
中国国家自然科学基金;
关键词
Photocatalysis; Bi2S3 ultrathin nanobelt; Oxygen-doped MoS2; Surface plasmon resonance; Photothermal effect; HYDROGEN EVOLUTION; G-C3N4; HETEROSTRUCTURES; DEGRADATION; NANOSHEETS; SYSTEM; CDS; FABRICATION; COMPOSITES; POLLUTANTS;
D O I
10.1016/j.apcatb.2020.118947
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Plasmon Ag nanoparticle/Bi2S3 ultrathin nanobelt/oxygen-doped flower-like MoS2 nanosphere ternary heterojunction photocatalysts are fabricated via hydrothermal and photoreduction strategies. The introduction of Ag nanoparticles and defective MoS2 and the formation of heterojunctions can induce localized surface plasmon resonance and promote charge separation, respectively, which can extend the photoresponse to the visible light and near-infrared regions and obviously enhance the photothermal and photocatalytic performances. The ternary heterojunction photocatalysts show that the photocatalytic degradation ratio of 2,4-dichlorophenol reaches 99.2% under visible light irradiation. In addition, the photocatalytic hydrogen evolution rate reaches 526.3 mu mol h(-1) g(-1), which is several times higher than that of pristine MoS2 and Bi2S3. This study offers a new strategy for designing other highly efficient heterojunction photocatalysts. In addition, these ternary heterojunctions show high stability, which is favorable for practical applications in the environmental and energy fields.
引用
收藏
页数:10
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