Investigation of photoelectrical properties of CdSe nanocrystals embedded in a SiO2 matrix

被引:7
作者
Kafadaryan, E. A. [1 ]
Levichev, S. [2 ]
Pinto, S. R. C. [2 ]
Aghamalyan, N. R. [1 ]
Hovsepyan, R. K. [1 ]
Badalyan, G. R. [1 ]
Chahboun, A. [2 ,3 ]
Rolo, A. G. [2 ]
Gomes, M. J. M. [2 ]
机构
[1] Natl Acad Sci, Inst Phys Res, Ashtarak 378410 2, Armenia
[2] Univ Minho, Dept Phys, P-4710057 Braga, Portugal
[3] Dhar El Mahraz Sci Fac, Dept Phys, LPS, Fes, Morocco
关键词
D O I
10.1088/0268-1242/23/9/095025
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
CdSe nanocrystals (NCs) embedded in SiO2 thin films were prepared using RF-magnetron co-sputtering. The average NC size was estimated to be 18 nm. The dark and photocurrent temporal dependences have been measured as a function of the magnitude of applied voltage (50-150 V). Annealing the samples seems to improve the photoconductivity (similar to 10(-12) Omega(-1)) that increases with the film thickness and slightly changes under the bias voltage. Furthermore, the photovoltage measurements showed that a concentration of CdSe in the range of 27 mol% leads to the generation of a photovoltaic signal up to 5 V at 400 mu W cm(-2). These results demonstrate the potential of silica films with embedded CdSe NCs for photovoltaic applications.
引用
收藏
页数:5
相关论文
共 21 条
[1]   Memory effects in optically active CdSe nanocrystal doped MOS structures [J].
Achtstein, A. W. ;
Karl, H. ;
Zhenhua, S. ;
Stritzker, B. .
MATERIALS SCIENCE AND ENGINEERING B-SOLID STATE MATERIALS FOR ADVANCED TECHNOLOGY, 2008, 147 (2-3) :249-253
[2]   Field induced photoluminescence quenching and enhancement of CdSe nanocrystals embedded in SiO2 [J].
Achtstein, A. W. ;
Karl, H. ;
Stritzker, B. .
APPLIED PHYSICS LETTERS, 2006, 89 (06)
[3]   Effect of substrate temperature and post-deposition annealing on the properties of evaporated CdSe thin films [J].
Bacaksiz, E. ;
Basol, B. M. ;
Altunbas, M. ;
Yilmaz, S. ;
Tomakin, M. ;
Abay, B. .
PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2007, 244 (02) :497-504
[4]   Percolative conduction in CdSe nanoparticles embedded in a silicon dioxide dielectric matrix [J].
Bera, SK ;
Chaudhuri, S ;
Pal, AK .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2000, 33 (18) :2320-2326
[5]   CdSe nanocrystal quantum-dot memory [J].
Fischbein, MD ;
Drndic, M .
APPLIED PHYSICS LETTERS, 2005, 86 (19) :1-3
[6]  
Gantmakher V. G., 2005, ELECT DISORDER SYSTE, P206
[7]   Percolation in transparent and conducting carbon nanotube networks [J].
Hu, L ;
Hecht, DS ;
Grüner, G .
NANO LETTERS, 2004, 4 (12) :2513-2517
[8]   Electrical, photo-electrical, optical and structural properties of CdSe thin films deposited by thermal and e-beam techniques [J].
Hus, S. M. ;
Parlak, M. .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2008, 41 (03)
[9]   QUANTUM-SIZE EFFECTS OF INTERACTING ELECTRONS AND HOLES IN SEMICONDUCTOR MICROCRYSTALS WITH SPHERICAL SHAPE [J].
KAYANUMA, Y .
PHYSICAL REVIEW B, 1988, 38 (14) :9797-9805
[10]   PERCOLATION AND CONDUCTION [J].
KIRKPATRICK, S .
REVIEWS OF MODERN PHYSICS, 1973, 45 (04) :574-588