Development of a Fully Integrated Micro-Scale Fuel Reformer over Platinum (Pt) Catalyst based on Low Temperature Co-Fired Ceramic (LTCC) Tape Technology

被引:0
作者
Huang, Chi-Mo [1 ]
Wang, Yi-Chun [1 ]
Wu, Ming-Hsun [1 ]
机构
[1] Natl Cheng Kung Univ, Dept Mech Engn, Tainan 701, Taiwan
来源
JOURNAL OF THE CHINESE SOCIETY OF MECHANICAL ENGINEERS | 2013年 / 34卷 / 03期
关键词
LTCC; Fuel reformer; Platinum; HYDROGEN-PRODUCTION; METHANOL; DECOMPOSITION; SYSTEM; CELLS; PROCESSOR; CERIA;
D O I
暂无
中图分类号
TH [机械、仪表工业];
学科分类号
0802 ;
摘要
Applying low temperature co-fired ceramic (LTCC) tape technology on constructing complex 3-D reacting flow and microfluidic devices has drawn increasing attention. In this paper, we developed a fully integrated micro-scale fuel reformer over Pt catalyst using LTCC tape technology, and we showed that the microfluidic channels and Pt catalytic layers in a LTCC reformer can be integrated by direct co-firing without additional processes. Current study also compared the effect of different thicknesses of Pt catalyst (10 and 40 nm) in LTCC reformers. As a source of hydrocarbon, methanol was used and the production of hydrocarbon fuels, including hydrogen, carbon monoxide and methane, was measured by gas chromatography. Among different parameters tested, our results revealed that a LTCC reformer coated with 10-nm Pt catalyst can generate most hydrocarbon fuels at a flow rate of 1 ml/h at a temperature of 300 degrees C. Overall, LTCC tape technology is a simple, reliable method to fabricate a fully integrated micro fuel reformer.
引用
收藏
页码:203 / 211
页数:9
相关论文
共 24 条
[1]   Hydrogen production from methanol decomposition over Pt/Al2O3 and ceria promoted Pt/Al2O3 catalysts [J].
Brown, JC ;
Gulari, E .
CATALYSIS COMMUNICATIONS, 2004, 5 (08) :431-436
[2]   Hydrogen production using integrated methanol-steam reforming reactor with various reformer designs for PEM fuel cells [J].
Chein, Rei-Yu ;
Chen, Yen-Cho ;
Lin, Yu-Sheng ;
Chung, J. N. .
INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2012, 36 (04) :466-476
[3]   A methanol steam micro-reformer for low power fuel cell applications [J].
Cominos, V ;
Hardt, S ;
Hessel, V ;
Kolb, G ;
Löwe, H ;
Wichert, M ;
Zapf, R .
CHEMICAL ENGINEERING COMMUNICATIONS, 2005, 192 (05) :685-698
[4]   Hydrogen from catalytic reforming of biomass-derived hydrocarbons in liquid water [J].
Cortright, RD ;
Davda, RR ;
Dumesic, JA .
NATURE, 2002, 418 (6901) :964-967
[5]  
Ghenciu AF, 2002, CURR OPIN SOLID ST M, V6, P389, DOI 10.1016/S1359-0286(02)00108-0
[6]   Overview of low temperature co-fired ceramics tape technology for meso-system technology (MsST) [J].
Gongora-Rubio, MR ;
Espinoza-Vallejos, P ;
Sola-Laguna, L ;
Santiago-Avilés, JJ .
SENSORS AND ACTUATORS A-PHYSICAL, 2001, 89 (03) :222-241
[7]   Review of developments in portable hydrogen production using microreactor technology [J].
Holladay, JD ;
Wang, Y ;
Jones, E .
CHEMICAL REVIEWS, 2004, 104 (10) :4767-4789
[8]   Decomposition of methanol on Pt-loaded ceria [J].
Imamura, S ;
Hagashihara, T ;
Saito, Y ;
Aritani, H ;
Kanai, H ;
Matsumura, Y ;
Tsuda, N .
CATALYSIS TODAY, 1999, 50 (02) :369-380
[9]   The effects of geometric and operating conditions on the hydrogen production performance of a micro-methanol steam reformer [J].
Jang, Jiin-Yuh ;
Huang, Yu-Xian ;
Cheng, Chin-Hsiang .
CHEMICAL ENGINEERING SCIENCE, 2010, 65 (20) :5495-5506
[10]   Micro-fuel cells - Current development and applications [J].
Kundu, Arunabha ;
Jang, J. H. ;
Gil, J. H. ;
Jung, C. R. ;
Lee, H. R. ;
Kim, S.-H. ;
Ku, B. ;
Oh, Y. S. .
JOURNAL OF POWER SOURCES, 2007, 170 (01) :67-78