De Novo Design of Nanostructured Iron-Cobalt Fischer-Tropsch Catalysts

被引:103
作者
Calderone, V. Roberto [1 ]
Shiju, N. Raveendran [1 ]
Curulla-Ferre, Daniel [2 ]
Chambrey, Stephane [3 ]
Khodakov, Andrei [3 ]
Rose, Amadeus [4 ]
Thiessen, Johannes [4 ]
Jess, Andreas [4 ]
Rothenberg, Gadi [1 ]
机构
[1] Univ Amsterdam, Vant Hoff Inst Mol Sci, NL-1098 XH Amsterdam, Netherlands
[2] Total SA, Gaz & Energies Nouvelles, Paris 6, France
[3] Univ Sci & Technol Lille 1, UCCS, F-59651 Villeneuve Dascq, France
[4] Univ Bayreuth, Ctr Energy Technol, Dept Chem Engn, D-95440 Bayreuth, Germany
关键词
cobalt; FischerTropsch synthesis; heterogeneous catalysis; nanoparticles; synthetic fuels; FE-CO/TIO2 BIMETALLIC CATALYSTS; FE-CO;
D O I
10.1002/anie.201209799
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Audio cassettes hold the key to enhancing Fischer-Tropsch catalysis. Catalysts based on ultra-thin cobalt shells surrounding cheap iron oxide cores (see picture) are developed, an approach previously optimized for preparing magnetic tape for audio cassettes. These particles are easily made on a large scale, and are excellent Fischer-Tropsch catalysts, giving good diesel fractions. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:4397 / 4401
页数:5
相关论文
共 29 条
  • [11] Fe:Co/TiO2 bimetallic catalysts for the Fischer-Tropsch reaction .1. Characterization and reactor studies
    Duvenhage, DJ
    Coville, NJ
    [J]. APPLIED CATALYSIS A-GENERAL, 1997, 153 (1-2) : 43 - 67
  • [12] European Commission, 2010, CRIT RAW MAT EU CAN
  • [13] Concerning the synthesis of upper links in the aliphatic sequence from carbon oxide.
    Fischer, F
    Tropsch, H
    [J]. BERICHTE DER DEUTSCHEN CHEMISCHEN GESELLSCHAFT, 1923, 56 : 2428 - 2443
  • [14] Haller W. D., 1971, [No title captured], Patent No. [US3573980, 3573980]
  • [15] CHARACTERISTICS OF COBALT ADSORBED IRON-OXIDE TAPES
    IMAOKA, Y
    UMEKI, S
    KUBOTA, Y
    TOKUOKA, Y
    [J]. IEEE TRANSACTIONS ON MAGNETICS, 1978, 14 (05) : 649 - 654
  • [16] Thermally stable Pt/mesoporous silica core-shell nanocatalysts for high-temperature reactions
    Joo, Sang Hoon
    Park, Jeong Young
    Tsung, Chia-Kuang
    Yamada, Yusuke
    Yang, Peidong
    Somorjai, Gabor A.
    [J]. NATURE MATERIALS, 2009, 8 (02) : 126 - 131
  • [17] Kanten T. M., 1980, [No title captured], Patent No. [US4226909, 4226909]
  • [18] Fischer-Tropsch synthesis: Relations between structure of cobalt catalysts and their catalytic performance
    Khodakov, Andrei Y.
    [J]. CATALYSIS TODAY, 2009, 144 (3-4) : 251 - 257
  • [19] Lehner A., 1982, [No title captured], Patent No. [US4328282, 4328282]
  • [20] Hydrocarbon production via Fischer-Tropsch synthesis from H2-poor syngas over different Fe-Co/γ-Al2O3 bimetallic catalysts
    Logdberg, Sara
    Tristantini, Dewi
    Borg, Oyvind
    Ilver, Lars
    Gevert, Boerje
    Jaras, Sven
    Blekkan, Edd A.
    Holmen, Anders
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2009, 89 (1-2) : 167 - 182