Weather Condition Dominates Regional PM2.5 Pollutions in the Eastern Coastal Provinces of China during Winter

被引:27
作者
Cai, Zhe [1 ,4 ]
Jiang, Fei [1 ,3 ]
Chen, Jingming [1 ,2 ]
Jiang, Ziqiang [1 ]
Wang, Xiaoyuan [5 ]
机构
[1] Nanjing Univ, Int Inst Earth Syst Sci, Jiangsu Prov Key Lab Geog Informat Sci & Technol, Nanjing 210023, Jiangsu, Peoples R China
[2] Univ Toronto, Dept Geog, Toronto, ON M5S 3G3, Canada
[3] Jiangsu Ctr Collaborat Innovat Geog Informat Reso, Nanjing 210023, Jiangsu, Peoples R China
[4] Jinan Meteorol Bur, Jinan 250102, Shandong, Peoples R China
[5] Zhejiang Environm Monitoring Ctr, Hangzhou 310015, Zhejiang, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金; 国家重点研发计划;
关键词
Weather condition; Regional PM2.5 pollution; China eastern coastal provinces; YANGTZE-RIVER DELTA; FOSSIL-FUEL COMBUSTION; HEAVY HAZE EVENTS; NORTH CHINA; AIR-QUALITY; SOURCE APPORTIONMENT; SYNOPTIC WEATHER; AEROSOL; IMPACT; EPISODE;
D O I
10.4209/aaqr.2017.04.0140
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
China has suffered from severe particulate matter (PM) pollution in recent years. Both pollution areas and levels are increasing gradually. The PM pollution episodes not only occur in the traditional developed areas like the Yangtze River Delta (YRD) and the Beijing-Tianjin-Hebei (BTH) region, but also frequently happen in the eastern coastal provinces (ECPs) of China. Based on hourly fine-PM (PM2.5) concentrations during December 2013 to February 2014 of 55 cities located in the ECPs, we investigated the spatial and temporal variabilities of PM2.5 concentration and the corresponding meteorological conditions during winter. The results generally showed that the winter mean concentrations over all ECPs exceeded China's national standard of 75 mu g m(-3), and the most polluted areas with mean concentrations exceeding 150 mu g m(-3) were in the southwest of Hebei and the west of Shandong Province. The PM2.5 concentrations in February were lower than December in most areas, especially in the YRD, but they were higher over the north of Hebei Province. The spatial distributions and monthly variations were strongly related to weather conditions. Overall, severe PM pollution corresponded with stable weather conditions: small Sea Level Pressure gradient, lower Planetary Boundary Layer (PBL) height and weaker winds. Statistics showed that the changes of the mean PM2.5 concentration over the ECP region lagged behind the variations in the PBL height and wind speeds by about 12-18 h, and the variations in weather conditions could explain about 71% (R-2) of the overall changes in PM2.5 concentrations, indicating that regional PM2.5 pollution was dominated by weather conditions in the ECPs. This study gives insight into the PM2.5 pollution in the ECPs of China during winter, which would be helpful to predict and control the PM2.5 pollution for this area in the future.
引用
收藏
页码:969 / 980
页数:12
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