Facile fabrication of highly efficient g-C3N4/BiFeO3 nanocomposites with enhanced visible light photocatalytic activities

被引:109
作者
Wang, Xingfu [1 ,2 ]
Mao, Weiwei [1 ,2 ]
Zhang, Jian [1 ]
Han, Yumin [1 ]
Quan, Chuye [1 ]
Zhang, Qiaoxia [1 ]
Yang, Tao [1 ]
Yang, Jianping [2 ]
Li, Xing'ao [1 ]
Huang, Wei [1 ,3 ,4 ]
机构
[1] NUPT, SMSE, IAM, KLOEID,SICOEID, Nanjing 210023, Jiangsu, Peoples R China
[2] NUPT, Sch Sci, Nanjing 210023, Jiangsu, Peoples R China
[3] Nanjing Tech Univ NanjingTech, Natl Synergist Innovat Ctr Adv Mat SICAM, Key Lab Flexible Elect KLOFE, Nanjing 211816, Jiangsu, Peoples R China
[4] Nanjing Tech Univ NanjingTech, IAM, Nanjing 211816, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
g-C3N4; BiFeO3; Nanocomposites; Photocatalysis; HYDROTHERMAL SYNTHESIS; HETEROJUNCTIONS; HYBRID; NANOPARTICLES; DEGRADATION; G-C3N4;
D O I
10.1016/j.jcis.2015.01.090
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Graphitic carbon nitride/bismuth ferrite (g-C3N4/BiFeO3) nanocomposites with various g-C3N4 contents have been synthesized by a simple method. After the deposition-precipitation process, the novel BiFeO3 spindle-like nanoparticles with the size of similar to 100 nm were homogeneously decorated on the surfaces of the C3N4 nanosheets. A possible deposition growth mechanism is proposed on the basis of experimental results. The as-prepared g-C3N4/BiFeO3 composites exhibit high efficiency for the degradation of methyl orange (MO) under visible light irradiation, which can be mainly attributed to the synergic effect between g-C3N4 and BiFeO3. The ability to tune surface and interfacial characteristics for the optimization of photophysical properties suggests that the deposition growth process may enable formation of hybrids suitable for a range of photocatalytic applications based on g-C3N4. (C) 2015 Elsevier Inc. All rights reserved.
引用
收藏
页码:17 / 23
页数:7
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