Evidence of Strong Correlations and Coherence-Incoherence Crossover in the Iron Pnictide Superconductor KFe2As2

被引:142
作者
Hardy, F. [1 ]
Boehmer, A. E. [1 ]
Aoki, D. [2 ,3 ]
Burger, P. [1 ]
Wolf, T. [1 ]
Schweiss, P. [1 ]
Heid, R. [1 ]
Adelmann, P. [1 ]
Yao, Y. X. [4 ]
Kotliar, G. [5 ]
Schmalian, J. [6 ]
Meingast, C. [1 ]
机构
[1] Karlsruher Inst Technol, Inst Festkorperphys, D-76021 Karlsruhe, Germany
[2] CEA Grenoble, INAC SPSMS, F-38054 Grenoble, France
[3] Tohoku Univ, IMR, Oarai, Ibaraki 3111313, Japan
[4] US DOE, Ames Lab, Ames, IA 50011 USA
[5] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA
[6] Karlsruher Inst Technol, Inst Theorie Kondensierten Mat, D-76128 Karlsruhe, Germany
关键词
TRANSITION; HEAT;
D O I
10.1103/PhysRevLett.111.027002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using resistivity, heat-capacity, thermal-expansion, and susceptibility measurements we study the normal-state behavior of KFe2As2. Both the Sommerfeld coefficient (gamma approximate to 103 mJ mol(-1) K-2) and the Pauli susceptibility (chi approximate to 4 x 10(-4)) are strongly enhanced, which confirm the existence of heavy quasiparticles inferred from previous de Haas-van Alphen and angle-resolved photoemission spectroscopy experiments. We discuss this large enhancement using a Gutzwiller slave-boson mean-field calculation, which shows the proximity of KFe2As2 to an orbital-selective Mott transition. The temperature dependence of the magnetic susceptibility and the thermal expansion provide strong experimental evidence for the existence of a coherence-incoherence crossover, similar to what is found in heavy fermion and ruthenate compounds, due to Hund's coupling between orbitals.
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页数:5
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